Oxford Centre for High Energy Density Science (OxCHEDS)

Abstract:

Bright high harmonic radiation from relativistically oscillating laser-plasmas offers a direct route to generating extreme electromagnetic fields. Theory shows that under optimised conditions the plasma medium can support strong spatiotemporal compression of laser energy into a Coherent Harmonic Focus (CHF), delivering intensity boosts many orders of magnitude above that of the incident driving laser pulse [1–4]. Although diffraction-limited performance [5] (spatial compression) and attosecond phase-locking [6] (temporal compression) have been demonstrated in the laboratory, efficient coupling of highly relativistic laser pulse energy into the emitted harmonic cone has not been realised to date. Here, conclusive evidence confirms that the relativistic laserplasma interaction can be tailored to deliver the maximum conversion efficiencies predicted from simulations. By fine-tuning the temporal profile of the driving laser pulse on femtosecond (fs, 10−15 s) timescales, energies > 9 mJ between the 12th and 47th harmonics (18 eV to 73 eV) are observed. These results are shown to be in excellent agreement with the theoretically expected efficiency dependence on harmonic order, indicating that optimal conditions have been achieved in the generation process. This is the important final element required to achieve the expected intensity boosts from a CHF in the laboratory. Although obtaining spatiotemporal compression and optimal efficiency simultaneously remains challenging, the path to realising extreme optical field strengths approaching the critical field of quantum electrodynamics (the Schwinger limit at > 1016V/m or > 1029 W cm−2 ) is now open, permitting all-optical studies of the quantum vacuum and drawing new horizons for intense attosecond science.

Abstract:

Bright harmonic radiation from relativistically oscillating laser plasmas offers a direct route for generating extreme electromagnetic fields. Theory predicts that under optimized conditions, the plasma medium can support strong spatiotemporal compression of laser energy in a coherent harmonic focus (CHF), delivering intensity boosts many orders of magnitude greater than the incident driving laser pulse^1,2,3,4. Although diffraction-limited performance⁵ (spatial compression) and attosecond phase locking^6,7,8 (temporal compression) have been demonstrated experimentally, efficient coupling of relativistically intense laser pulse energy into the emitted harmonic cone has not been realized so far. Here we demonstrate that this highly nonlinear interaction can be tailored to deliver the maximum conversion efficiencies predicted from simulations. By fine-tuning the temporal profile of the driving laser on sub-picosecond (<10⁻¹² s) timescales, energies >9 mJ between the 12th and 47th harmonics are observed. These results are in agreement with the theoretically expected efficiency dependence on harmonic order, verifying that optimal conditions have been achieved in the generation process. This is the important final element required to achieve the expected intensity boosts from a CHF in experiments. Although obtaining spatiotemporal compression and optimal efficiency simultaneously remains challenging, the path to realizing extreme optical field strengths approaching the critical field of quantum electrodynamics (the Schwinger limit at >10¹⁶ V cm⁻¹ or >10²⁹ W cm⁻²) is now open, permitting all-optical studies of the quantum vacuum and new frontiers for intense attosecond science.