Formation of nucleobases in a Miller-Urey reducing atmosphere.

Proceedings of the National Academy of Sciences of the United States of America 114:17 (2017) 4306-4311

Authors:

Martin Ferus, Fabio Pietrucci, Antonino Marco Saitta, Antonín Knížek, Petr Kubelík, Ondřej Ivanek, Violetta Shestivska, Svatopluk Civiš

Abstract:

The Miller-Urey experiments pioneered modern research on the molecular origins of life, but their actual relevance in this field was later questioned because the gas mixture used in their research is considered too reducing with respect to the most accepted hypotheses for the conditions on primordial Earth. In particular, the production of only amino acids has been taken as evidence of the limited relevance of the results. Here, we report an experimental work, combined with state-of-the-art computational methods, in which both electric discharge and laser-driven plasma impact simulations were carried out in a reducing atmosphere containing NH3 + CO. We show that RNA nucleobases are synthesized in these experiments, strongly supporting the possibility of the emergence of biologically relevant molecules in a reducing atmosphere. The reconstructed synthetic pathways indicate that small radicals and formamide play a crucial role, in agreement with a number of recent experimental and theoretical results.

Spontaneous oxygen isotope exchange between carbon dioxide and natural clays: Refined rate constants referenced to TiO2 (anatase/rutile)

Applied Clay Science Elsevier BV 137 (2017) 6-10

Authors:

Antonín Knížek, Markéta Zukalová, Ladislav Kavan, Arnošt Zukal, Petr Kubelík, Petr Rojík, Petr Skřehot, Martin Ferus, Svatopluk Civiš

Introduction to the SPARC Reanalysis Intercomparison Project (S-RIP) and overview of the reanalysis systems

Atmospheric Chemistry and Physics Copernicus Publications 17:2 (2017) 1417-1452

Authors:

Masatomo Fujiwara, Jonathon S Wright, Gloria L Manney, Lesley J Gray, James Anstey, Thomas Birner, Sean Davis, Edwin P Gerber, V Lynn Harvey, Michaela I Hegglin, Cameron R Homeyer, John A Knox, Kirstin Krüger, Alyn Lambert, Craig S Long, Patrick Martineau, Andrea Molod, Beatriz M Monge-Sanz, Michelle L Santee, Susann Tegtmeier, Simon Chabrillat, David GH Tan, David R Jackson, Saroja Polavarapu, Gilbert P Compo, Rossana Dragani, Wesley Ebisuzaki, Yayoi Harada, Chiaki Kobayashi, Will McCarty, Kazutoshi Onogi, Steven Pawson, Adrian Simmons, Krzysztof Wargan, Jeffrey S Whitaker, Cheng-Zhi Zou

Retrieval of ash properties from IASI measurements

ATMOSPHERIC MEASUREMENT TECHNIQUES 9:11 (2016) 5407-5422

Authors:

LJ Ventress, G McGarragh, E Carboni, AJ Smith, RG Grainger

Simulation of stratospheric ozone in global forecast model using linear photochemistry parameterization

Asia-Pacific Journal of Atmospheric Sciences Springer Nature 52:5 (2016) 479-494

Authors:

Gill-Ran Jeong, Beatriz M Monge-Sanz, Eun-Hee Lee, Jerald R Ziemke