Laser fusion and extreme field physics

Abstract:

Laser peak powers rise inexorably higher, enabling the study of increasingly exotic high-energy-density plasmas. This thesis explores one such phenomenon, that of the interaction between a relativistically intense laser pulse and a solid-density plasma. The laser pulse is reflected. Both the reflected radiation and the electron bunches that induce the interaction have fascinating properties. Through the application of theory, simulation and experiment, this thesis strives to extend our understanding of this mechanism and thus direct the community towards potential applications for these sources. Of primary interest is the development of novel diagnostic tools. Theories have been developed and tested to describe the production of low emittance nano-Coulomb charge electron bunches. Such properties are comparable to forefront synchrotron sources but on a considerably more compact scale. These results have wide-reaching implications for future particle accelerator science and associated technologies. Furthermore, these electron bunches will initiate QED processes on next-generation laser facilities. The radiation they produce is composed of high harmonics of the incident laser pulse. This radiation can be coherently focused to unprecedented intensities and is of ultra-short duration, possibly even entering the zeptosecond regime. The intensity of X-ray harmonics has been measured on the ORION laser facility producing results consistent with theory and enabling the benchmarking of peak intensity simulations with real data. The work of this thesis has amassed interest within the community and in June 2024 its ideas will be tested on the GEMINI PW laser facility.

Abstract:

The optimisation of laser pulse shapes and target configurations is central to high-performance inertial confinement fusion (ICF) implosions, yet remains challenging due to the high dimensionality of the design space and the substantial computational and experimental cost of evaluation. This work presents, to our knowledge, the first comparison of GP-based Bayesian optimisation and particle swarm optimisation (PSO) frameworks augmented with physics-motivated extensions in full radiation-hydrodynamic ICF optimisation under experimentally relevant constraint handling. These methods are first applied to the reoptimisation of low-convergence-ratio (Low-CR) wetted-foam implosions, providing a benchmark against traditional sequential scan approaches. Both strategies identify improved designs, with Bayesian optimisation achieving the highest final performance using fewer simulations, while PSO converges more rapidly in wall-clock time. The PSO framework is then extended to a 16-dimensional fast ignition design problem, where Gaussian process-based Bayesian optimisation becomes computationally impractical. In this regime, PSO efficiently identifies a compressed fuel assembly with ρR ≈ 1.5 g/cm2 under strict laser intensity and energy constraints. These results demonstrate that the presented optimisation strategies outperform conventional scan-based approaches and provide a scalable platform for high-dimensional ICF optimisation. Beyond numerical design studies, the same frameworks are directly applicable to experimental optimisation campaigns on high-power laser facilities, where limited shot availability and high evaluation cost demand efficient search methodologies.

Abstract:

Inertial confinement fusion fuel suffers increased X-ray radiation losses when carbon from the capsule ablator mixes into the hot-spot. Here we present one and two-dimensional ion VlasovFokker-Planck simulations that resolve hot-spot self heating in the presence a localised spike of carbon mix, totalling 1.9 % of the hot-spot mass. The mix region cools and contracts over tens of picoseconds, increasing its alpha particle stopping power and radiative losses. This makes a localised mix region more severe than an equal amount of uniformly distributed mix. There is also a purely kinetic effect that reduces fusion reactivity by several percent, since faster ions in the tail of the distribution are absorbed by the mix region. Radiative cooling and contraction of the spike induces fluid motion, causing neutron spectrum broadening. This artificially increases the inferred experimental ion temperatures and gives line of sight variations.

Abstract:

The orbital angular momentum (OAM) of light is one of the most intriguing properties of electromagnetic radiation. Although OAM is more commonly associated with the mechanical movement of massive particles, researchers have shown that, under certain conditions, laser beams can carry it. This is not merely a theoretical proposition, this idea was almost immediately experimentally proven by showing that OAM can be transferred between light and matter. This has, in turn, spurred an ever-increasing interest in leveraging the interesting proprieties of the OAM of light for various technological applications. This work focuses on the effect that OAM has on high-intensity laser interactions.

High-intensity lasers have been a boon to scientific investigations in their own right. They have allowed us to experimentally research astrophysical phenomena inside of laboratories, opened the possibility to tabletop particle accelerators and gotten us closer to useful fusion energy sources. More recently, we have been able to reach extreme intensities that allow us to probe the most fundamental interactions in the universe. Predictions that had been theorized decades ago by the pioneers of the quantum theory of matter are now close to being experimentally verifiable.

In the coming chapters, I look at the fundamental nature of the OAM of light and the many discussions it has spurred. I then show that it modifies an interaction known as vacuum photon-photon scattering where beams of light can interact with each other in the absence of any mediating matter violating the constraints established by the classical theory of electromagnetism. OAM provides an extra signal that makes this light-light interaction more identifiable in an experiment. On a more practical note, I continue to look specifically at high-intensity lasers and how they can be manipulated to produce high-intensity OAM-carrying beams and how said beams can be characterized.

Abstract:

Bright high harmonic radiation from relativistically oscillating laser-plasmas offers a direct route to generating extreme electromagnetic fields. Theory shows that under optimised conditions the plasma medium can support strong spatiotemporal compression of laser energy into a Coherent Harmonic Focus (CHF), delivering intensity boosts many orders of magnitude above that of the incident driving laser pulse [1–4]. Although diffraction-limited performance [5] (spatial compression) and attosecond phase-locking [6] (temporal compression) have been demonstrated in the laboratory, efficient coupling of highly relativistic laser pulse energy into the emitted harmonic cone has not been realised to date. Here, conclusive evidence confirms that the relativistic laserplasma interaction can be tailored to deliver the maximum conversion efficiencies predicted from simulations. By fine-tuning the temporal profile of the driving laser pulse on femtosecond (fs, 10−15 s) timescales, energies > 9 mJ between the 12th and 47th harmonics (18 eV to 73 eV) are observed. These results are shown to be in excellent agreement with the theoretically expected efficiency dependence on harmonic order, indicating that optimal conditions have been achieved in the generation process. This is the important final element required to achieve the expected intensity boosts from a CHF in the laboratory. Although obtaining spatiotemporal compression and optimal efficiency simultaneously remains challenging, the path to realising extreme optical field strengths approaching the critical field of quantum electrodynamics (the Schwinger limit at > 1016V/m or > 1029 W cm−2 ) is now open, permitting all-optical studies of the quantum vacuum and drawing new horizons for intense attosecond science.