Philip Stier

Abstract:

A multi-agency succession of field campaigns was conducted in southeastern Texas during July 2021 through October 2022 to study the complex interactions of aerosols, clouds and air pollution in the coastal urban environment. As part of the Tracking Aerosol Convection interactions Experiment (TRACER), the TRACER- Air Quality (TAQ) campaign the Experiment of Sea Breeze Convection, Aerosols, Precipitation and Environment (ESCAPE) and the Convective Cloud Urban Boundary Layer Experiment (CUBE), a combination of ground-based supersites and mobile laboratories, shipborne measurements and aircraft-based instrumentation were deployed. These diverse platforms collected high-resolution data to characterize the aerosol microphysics and chemistry, cloud and precipitation micro- and macro-physical properties, environmental thermodynamics and air quality-relevant constituents that are being used in follow-on analysis and modeling activities. We present the overall deployment setups, a summary of the campaign conditions and a sampling of early research results related to: (a) aerosol precursors in the urban environment, (b) influences of local meteorology on air pollution, (c) detailed observations of the sea breeze circulation, (d) retrieved supersaturation in convective updrafts, (e) characterizing the convective updraft lifecycle, (f) variability in lightning characteristics of convective storms and (g) urban influences on surface energy fluxes. The work concludes with discussion of future research activities highlighted by the TRACER model-intercomparison project to explore the representation of aerosol-convective interactions in high-resolution simulations.

Abstract:

Anthropogenic aerosols are a primary source of uncertainty in future climate projections. Changes to aerosol concentrations modify cloud radiative properties, radiative fluxes, and precipitation from the micro- to the global scale. Due to computational constraints, we have been unable to explicitly simulate cloud dynamics in global-scale simulations, leaving key processes, such as convective updrafts, parameterized. This has significantly limited our understanding of aerosol impacts on convective clouds and climate. However, new state-of-the-art climate models are capable of representing these scales. In this study, we used the kilometer-scale Icosahedral Nonhydrostatic (ICON) earth system model to explore the global-scale rapid response of clouds and precipitation to an idealized distribution of anthropogenic aerosol via aerosol-cloud interactions (ACI) and aerosol-radiation interactions (ARI). In our simulations over 30 days, we find that the aerosol impacts on clouds and precipitation exhibit strong regional dependence. The impact of ARI and ACI on clouds in isolation shows some consistent behavior, but the magnitude and additive nature of the effects are regionally dependent. Some regions are dominated by either ACI or ARI, whereas others behaved nonlinearly. This suggests that the findings of isolated case studies from regional simulations may not be globally representative; ARI and ACI cannot be considered independently and should both be interactively represented in modelling studies. We also observe pronounced diurnal cycles in the rapid response of cloud microphysical and radiative properties, which suggests the usefulness of using polar-orbiting satellites to quantify ACI and ARI may be more limited than presently assumed. The simulations highlight some limitations that need to be considered in future studies. Isolating kilometerscale aerosol responses from internal variability will require longer averaging periods or ensemble simulations. It would also be beneficial to use interactive aerosols and assess the sensitivity of the conclusions to the cloud microphysics scheme.

Abstract:

Anthropogenic emissions of black carbon (BC) aerosols are generally thought to warm the climate. However, the magnitude of this warming remains highly uncertain due to limited knowledge of BC sources; optical properties; and atmospheric processes such as transport, removal, and cloud interactions. Here, we assess and constrain estimates of the historical warming influence of BC using recent observations and emission inventories. Based on simulations from four climate models, we show that the current global mean surface temperature change from anthropogenic BC due to aerosol-radiation interaction spans a factor of three—from +0.02 ± 0.02 K to +0.06 ± 0.05 K. Rapid atmospheric adjustments reduce the instantaneous radiative forcing by nearly 50% (multi-model mean), substantially lowering the net warming. Yet, recent satellite constraints suggest a stronger effect, highlighting the need for a more comprehensive reassessment of BC’s climate influence.

Abstract:

Realistically representing deep atmospheric convection is important for accurate numerical weather and climate simulations. However, parameterizing where and when deep convection occurs (“triggering”) is a well-known source of model uncertainty. Most triggers parameterize convection deterministically, without considering the uncertainty in the convective state as a stochastic process. In this study, we develop a machine learning model, a random forest, that predicts the probability of deep convection, and then apply clustering of SHAP values, an explainable machine learning method, to characterize the uncertainty of convective events. The model uses observed large-scale atmospheric variables from the Atmospheric Radiation Measurement constrained variational analysis dataset over the Southern Great Plains, US. The analysis of feature importance shows which mechanisms driving convection are most important, with large-scale vertical velocity providing the highest predictive power for more certain, or easier to predict, convective events, followed by the dynamic generation rate of dilute convective available potential energy. Predictions of uncertain, or harder to predict, convective events instead rely more on other features such as precipitable water or low-level temperature. The model outperforms conventional convective triggers. This suggests that probabilistic machine learning models can be used as stochastic parameterizations to improve the occurrence of convection in weather and climate models in the future.