Regional and monthly and clear-sky aerosol direct radiative effect (and forcing) derived from the GlobAEROSOL-AATSR satellite aerosol product

Atmospheric Chemistry and Physics 13:1 (2013) 393-410

Authors:

GE Thomas, N Chalmers, B Harris, RG Grainger, EJ Highwood

Abstract:

Using the GlobAEROSOL-AATSR dataset, estimates of the instantaneous, clear-sky, direct aerosol radiative effect and radiative forcing have been produced for the year 2006. Aerosol Robotic Network sun-photometer measurements have been used to characterise the random and systematic error in the GlobAEROSOL product for 22 regions covering the globe. Representative aerosol properties for each region were derived from the results of a wide range of literature sources and, along with the de-biased GlobAEROSOL AODs, were used to drive an offline version of the Met Office unified model radiation scheme. In addition to the mean AOD, best-estimate run of the radiation scheme, a range of additional calculations were done to propagate uncertainty estimates in the AOD, optical properties, surface albedo and errors due to the temporal and spatial averaging of the AOD fields. This analysis produced monthly, regional estimates of the clear-sky aerosol radiative effect and its uncertainty, which were combined to produce annual, global mean values of (-6.7 ± 3.9) W m-2 at the top of atmosphere (TOA) and (-12 ± 6) W m-2 at the surface. These results were then used to give estimates of regional, clear-sky aerosol direct radiative forcing, using modelled pre-industrial AOD fields for the year 1750 calculated for the AEROCOM PRE experiment. However, as it was not possible to quantify the uncertainty in the pre-industrial aerosol loading, these figures can only be taken as indicative and their uncertainties as lower bounds on the likely errors. Although the uncertainty on aerosol radiative effect presented here is considerably larger than most previous estimates, the explicit inclusion of the major sources of error in the calculations suggest that they are closer to the true constraint on this figure from similar methodologies, and point to the need for more, improved estimates of both global aerosol loading and aerosol optical properties. © 2013 Author(s).

Measuring volcanic plume and ash properties from space

Geological Society, London, Special Publications Geological Society of London 380:1 (2013) 293-320

Authors:

RG Grainger, DM Peters, GE Thomas, AJA Smith, R Siddans, E Carboni, A Dudhia

Abstract:

Abstract The remote sensing of volcanic ash plumes from space can provide a warning of an aviation hazard and knowledge on eruption processes and radiative effects. In this paper new algorithms are presented to provide volcanic plume properties from measurements by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS), the Advanced Along Track Scanning Radiometer (AATSR) and the Spinning Enhanced Visible and Infrared Imager (SEVIRI). A challenge of remote sensing is to provide near-real-time methods to identify, and so warn of, the presence of volcanic ash. To achieve this, a singular vector decomposition method has been developed for the MIPAS instrument on board the Environmental Satellite. This method was applied to observations of the ash clouds from the eruptions of Nabro and the Puyehue–Cordón Caulle in 2011 and led to a sensitive volcanic signal flag which was capable of tracking changes in the volcanic signal spectra as the plume evolved. A second challenge for remote sensing is to identify the ash plume height. This is a critical parameter for the initialization of algorithms that numerically model the evolution and transport of a volcanic plume. As MIPAS is a limb sounder, the identification of ash also provides an estimate of height provided the plume is above about 6 km. This is complemented by a new algorithm, Stereo Ash Plume Height Retrieval Algorithm, that identifies plume height using the parallax between images provided by Along Track Scanning Radiometer-type instruments. The algorithm was tested on an image taken at 14:01 GMT on 6 June 2011 of the Puyehue–Cordón Caulle eruption plume and gave a height of 11.9±1.4 km, which agreed with the value derived from the location of the plume shadow (12.7±1.8 km). This plume height was similar to the height observed by MIPAS (12 ± 1.5 km) at 02:56 GMT on 6 June. The quantitative use of satellite imagery and the full exploitation of high-resolution spectral measurements of ash depends upon knowing the optical properties of the observed ash. Laboratory measurements of ash from the 1993 eruption of Mt Aso, Japan have been used to determine the refractive indices from 1 to 20 µm. These preliminary measurements have spectral features similar to ash values that have been used to date, albeit with slightly different positions and strengths of the absorption bands. The refractive indices have been used to retrieve ash properties (plume height, optical depth and ash effective radius) from AATSR and SEVIRI instruments using two versions of Oxford-RAL Retrieval of Aerosol and Cloud (ORAC) algorithm. For AATSR a new ash cloud type was used in ORAC for the analysis of the plume from the 2011 Eyjafjallajökull eruption. For the first c . 500 km of the plume ORAC gave values for plume height of 2.5–6.5 km, optical depth 1–2.5 and effective radius 3–7 µm, which are in agreement with other observations. A weakness of the algorithm occurs when underlying cloud invalidates the assumption of a single cloud layer. This is rectified in a modified version of ORAC applied to SEVIRI measurements. In this case an extra model of a cloud underlying the ash plume was included in the range of applied models. In cases where the plume overlay cloud, this new model worked well, showing good agreement with correlative Cloud–Aerosol Lidar with Orthogonal Polarization observations.

A new scheme for sulphur dioxide retrieval from IASI measurements: application to the Eyjafjallajökull eruption of April and May 2010

Atmospheric Chemistry and Physics Copernicus Publications 12:23 (2012) 11417-11434

Authors:

E Carboni, R Grainger, J Walker, A Dudhia, R Siddans

Stratospheric aerosol particles and solar-radiation management

Nature Climate Change 2:10 (2012) 713-719

Authors:

FD Pope, P Braesicke, RG Grainger, M Kalberer, IM Watson, PJ Davidson, RA Cox

Abstract:

The deliberate injection of particles into the stratosphere has been suggested as a possible geoengineering scheme to mitigate the global warming aspect of climate change. Injected particles scatter solar radiation back to space and thus reduce the radiative balance of Earth. Previous studies investigating this scheme have focused primarily on sulphuric acid particles to mimic volcanic injections of stratospheric aerosol. However, the composition and size of volcanic sulphuric acid particles are far from optimal for scattering solar radiation. We show that aerosols with other compositions, such as minerals, could be used to dramatically increase the amount of light scatter achieved on a per mass basis, thereby reducing the particle mass required for injection. The chemical consequences of injecting such particles into the stratosphere are discussed with regard to the fate of the ozone layer. Research questions are identified with which to assess the feasibility of such geoengineering schemes. © 2012 Macmillan Publishers Limited. All rights reserved.

Estimation of a lidar's overlap function and its calibration by nonlinear regression

Applied Optics 51:21 (2012) 5130-5143

Authors:

AC Povey, RG Grainger, DM Peters, JL Agnew, D Rees

Abstract:

The overlap function of a Raman channel for a lidar system is retrieved by nonlinear regression using an analytic description of the optical system and a simple model for the extinction profile, constrained by aerosol optical thickness. Considering simulated data, the scheme is successful even where the aerosol profile deviates significantly from the simple model assumed. Applicationto real dataisfound to reduce by a factor of 1.4-2.0 the root-mean-square difference between the attenuated backscatter coefficient as measured by the calibrated instrument and a commercial instrument. © 2012 Optical Society of America.