Professor Roy Grainger

Abstract:

The cryogenic limb array etalon spectrometer (CLAES) and the improved stratospheric and mesospheric sounder (ISAMS) instruments on board the Upper Atmosphere Research Satellite (UARS) have been used to produce global information on the Mt. Pinatubo volcanic aerosol for the period from October 1991 to April 1993, The Satellite infrared extinction measurements near 12 mu m are converted into the aerosol-related parameters necessary for modelling the effects of the volcanic aerosol on the aeronomy of the stratosphere and are presented as zonal mean distributions for 80 degrees S to 80 degrees N averaged over similar to 35-day periods. The aerosol composition is derived from the CLAES and ISAMS temperature measurements and the water vapour abundances are obtained from the microwave limb sounder (MLS). The aerosol volume density is obtained from the extinction measurements from which the Surface area density and the effective particle radius are estimated. The maximum aerosol surface area density has a value of about 50 mu m(2) cm(-3) at a height of 24 km at the equator in October 1991, before decaying exponentially with a time constant of 443 +/- 10 days. The surface area density remained well above preeruption values in April 1993. The effective particle radius in the tropics decays monotonically from 0.65 mu m in October 1991 to 0.4 mu m in April 1993. The global aerosol sulphate mass loading is 19.5 Mt in October 1991 and decays exponentially with a time constant of 342 +/- 8 days to a value of 4.3 Mt by April 1993. Four months after the eruption the calculated optical thickness at 1.02 mu m was similar to 0.25 in the tropics. Rate constants are derived for the heterogeneous reactions of N2O5 and ClONO2 on the sulphate aerosols. The application of the aerosol parameters to the investigation of tracer transport, heterogeneous chemistry, and radiative transfer is discussed.

Abstract:

This paper introduces a series of papers describing the validation of data products from the improved stratospheric and mesospheric sounder (ISAMS) on the Upper Atmosphere Research Satellite. ISAMS is a limb-sounding infrared gas-correlation radiometer, measuring thermal emission from a range of constituents. The constituents measured are ozone, water vapor, methane, nitrous oxide, nitric oxide, nitrogen dioxide, nitrogen pentoxide, nitric acid, carbon monoxide, and aerosol. Atmospheric temperature and composition data were obtained for approximately 180 days between September 26, 1991, and July 29, 1992, with near-global coverage. The instrument and the retrieval process are briefly described, together with aspects of the validation process relevant to all data products, including the radiometric calibration and the analysis of the calibrated radiances to produce data on a standard time-altitude grid.

Abstract:

The improved stratospheric and mesospheric sounder (ISAMS) made ozone measurements in the stratosphere and mesosphere, with dense coverage over a broad range of latitudes, on about 180 days between September 1991 and July 1992. In this paper we are concerned with version 10 of the ISAMS data, which is recommended for use in the pressure range 10-0.1 mbar at night and 10-1 mbar during daytime. We describe the measurements and the retrieval algorithm, present an error analysis, and provide comparisons of the results to both climatological and coincident data. It is demonstrated that biases with respect to other well-validated data sets are less than 10%, which is well within the internal assessment of systemetic errors.

Abstract:

The retrieval and validation of the infrared measurements of the stratospheric aerosol layer derived from the improved stratospheric and mesospheric sounder (ISAMS) on board the Upper Atmsophere Research Satellite (UARS) are discussed in detail. The retrieval method is presented and an error analysis and sensitivity study are used to provide an error budget. The validation involves internal consistency checks, comparisons with coincident aerosol observations from other satellite-based instruments (cryogenic limb array etalon spectrometer (CLAES) and Stratospheric Aerosol and Gas Experiment II (SAGE II)) and in situ particle counters. The internal comparisons show that the precision of the 6.20-mu m retrievals are better than 30% for the data on the 32-hPa and 22-hPa pressure surfaces and that the 12.11-mu m retrievals are better than 20% and 25% for the data on pressure surfaces at 46 hPa and 32 hPa, respectively. Comparison of the ISAMS aerosol extinctions with the simultaneous CLAES measurements show systematic biases for both the 6-mu m and the 12-mu m retrievals with ISAMS generally measuring lower extinction values than CLAES. The comparison with calculated extinctions from balloon dustsonde data at 41 degrees N shows that the aerosol extinctions are systematically too high for pressures less than 40 hPa.

Abstract:

Results for the residual circulation in the stratosphere and lower mesosphere between September 1991 and August 1994 are reported. This circulation is diagnosed by applying an accurate radiative transfer code to temperature, ozone, and water vapor measurements acquired by the Microwave Limb Sounder (MLS) onboard the Upper Atmosphere Research Satellite (UARS), augmented by climatological distributions of methane, nitrous oxide, nitrogen dioxide, surface albedo, and cloud cover. The sensitivity of the computed heating rates to the presence of Mt. Pinatubo aerosols is explored by utilizing aerosol properties derived from the measurements obtained by the Improved Stratospheric and Mesospheric Sounder instrument, also onboard UARS. The computed vertical velocities exhibit a semiannual oscillation (SAG) around the tropical stratopause, with the region of downward velocities reaching maximum spatial extent in February and August. This behavior reflects the semiannual oscillation in temperature and ozone and mimics that seen in past studies of the October 1978-May 1979 period based on data from the Limb Infrared Monitor of the Stratosphere onboard the Nimbus 7 satellite. The SAO vertical velocities are stronger during the northern winter phase, as expected if planetary waves from the winter hemisphere are involved in driving the SAG. A possible quasi-biennial oscillation (QBO) signal extending from the middle into the upper stratosphere is also hinted at, with the equatorial vertical velocities in the region 10-1 hPa significantly smaller (or even negative) in 1993/94 than in 1992/93. Despite the short data record, the authors believe that this pattern reflects a QBO signal rather than a coincidental interannual variability, since the time-height section of vertical velocity at the equator resembles that of the zonal wind. Wintertime high-latitude descent rates are usually greater in the Northern Hemisphere, but they also exhibit significant variability there. In the three northern winters analyzed in this study, strong downward velocities are diagnosed in the lower stratosphere during stratospheric warmings and are associated with enhanced wave forcing (computed as the momentum residual) in the mid- and upper stratosphere. The implications of the computed circulation for the distribution of tracers are illustrated by the example of the ”double-peaked” structure in the water vapor distribution measured by MLS.