Satellite-derived sulfur dioxide (SO2) emissions from the 2014–2015 Holuhraun eruption (Iceland)

Atmospheric Chemistry and Physics Copernicus Publications 19 (2019) 4851-4862

Authors:

Elisa Carboni, Tamsin Mather, A Schmidt, Roy Grainger, MA Pfeffer, I Ialongo, N Theys

Abstract:

The 6-month-long 2014–2015 Holuhraun eruption was the largest in Iceland for 200 years, emitting huge quantities of sulfur dioxide (SO2) into the troposphere, at times overwhelming European anthropogenic emissions. Weather, terrain and latitude made continuous ground-based or UV satellite sensor measurements challenging. Infrared Atmospheric Sounding Interferometer (IASI) data are used to derive the first time series of daily SO2 mass present in the atmosphere and its vertical distribution over the entire eruption period. A new optimal estimation scheme is used to calculate daily SO2 fluxes and average e-folding time every 12 h. For the 6 months studied, the SO2 flux was observed to be up to 200 kt day−1 and the minimum total SO2 erupted mass was 4.4 ± 0.8 Tg. The average SO2 e-folding time was 2.4 ± 0.6 days. Where comparisons are possible, these results broadly agree with ground-based near-source measurements, independent remote-sensing data and values obtained from model simulations from a previous paper. The results highlight the importance of using high-resolution time series data to accurately estimate volcanic SO2 emissions. The SO2 mass missed due to thermal contrast is estimated to be of the order of 3 % of the total emission when compared to measurements by the Ozone Monitoring Instrument. A statistical correction for cloud based on the AVHRR cloud-CCI data set suggested that the SO2 mass missed due to cloud cover could be significant, up to a factor of 2 for the plume within the first kilometre from the vent. Applying this correction results in a total erupted mass of 6.7±0.4 Tg and little change in average e-folding time. The data set derived can be used for comparisons to other ground- and satellite-based measurements and to petrological estimates of the SO2 flux. It could also be used to initialise climate model simulations, helping to better quantify the environmental and climatic impacts of future Icelandic fissure eruptions and simulations of past large-scale flood lava eruptions.

Satellite-derived sulfur dioxide (SO2) emissions from the 2014–2015 Holuhraun eruption (Iceland)

Atmospheric Chemistry and Physics Copernicus Publications 19:7 (2019) 4851-4862

Authors:

Elisa Carboni, Tamsin A Mather, Anja Schmidt, Roy G Grainger, Melissa A Pfeffer, Iolanda Ialongo, Nicolas Theys

Abstract:

The 6-month-long 2014–2015 Holuhraun eruption was the largest in Iceland for 200 years, emitting huge quantities of sulfur dioxide (SO2) into the troposphere, at times overwhelming European anthropogenic emissions. Weather, terrain and latitude made continuous ground-based or UV satellite sensor measurements challenging. Infrared Atmospheric Sounding Interferometer (IASI) data are used to derive the first time series of daily SO2 mass present in the atmosphere and its vertical distribution over the entire eruption period. A new optimal estimation scheme is used to calculate daily SO2 fluxes and average e-folding time every 12 h. For the 6 months studied, the SO2 flux was observed to be up to 200 kt day−1 and the minimum total SO2 erupted mass was 4.4±0.8 Tg. The average SO2 e-folding time was 2.4±0.6 days. Where comparisons are possible, these results broadly agree with ground-based near-source measurements, independent remote-sensing data and values obtained from model simulations from a previous paper. The results highlight the importance of using high-resolution time series data to accurately estimate volcanic SO2 emissions. The SO2 mass missed due to thermal contrast is estimated to be of the order of 3 % of the total emission when compared to measurements by the Ozone Monitoring Instrument. A statistical correction for cloud based on the AVHRR cloud-CCI data set suggested that the SO2 mass missed due to cloud cover could be significant, up to a factor of 2 for the plume within the first kilometre from the vent. Applying this correction results in a total erupted mass of 6.7±0.4 Tg and little change in average e-folding time. The data set derived can be used for comparisons to other ground- and satellite-based measurements and to petrological estimates of the SO2 flux. It could also be used to initialise climate model simulations, helping to better quantify the environmental and climatic impacts of future Icelandic fissure eruptions and simulations of past large-scale flood lava eruptions.

SEAS5: the new ECMWF seasonal forecast system

Geoscientific Model Development European Geosciences Union 12:3 (2019) 1087-1117

Authors:

SJ Johnson, TN Stockdale, L Ferranti, MA Balmaseda, F Molteni, L Magnusson, S Tietsche, D Decremer, Antje Weisheimer, G Balsamo, SPE Keeley, K Mogensen, H Zuo, BM Monge-Sanz

Abstract:

In this paper we describe SEAS5, ECMWF's fifth generation seasonal forecast system, which became operational in November 2017. Compared to its predecessor, System 4, SEAS5 is a substantially changed forecast system. It includes upgraded versions of the atmosphere and ocean models at higher resolutions, and adds a prognostic sea-ice model. Here, we describe the configuration of SEAS5 and summarise the most noticeable results from a set of diagnostics including biases, variability, teleconnections and forecast skill.

An important improvement in SEAS5 is the reduction of the equatorial Pacific cold tongue bias, which is accompanied by a more realistic El Niño amplitude and an improvement in El Niño prediction skill over the central-west Pacific. Improvements in 2 m temperature skill are also clear over the tropical Pacific. Sea-surface temperature (SST) biases in the northern extratropics change due to increased ocean resolution, especially in regions associated with western boundary currents. The increased ocean resolution exposes a new problem in the northwest Atlantic, where SEAS5 fails to capture decadal variability of the North Atlantic subpolar gyre, resulting in a degradation of DJF 2 m temperature prediction skill in this region. The prognostic sea-ice model improves seasonal predictions of sea-ice cover, although some regions and seasons suffer from biases introduced by employing a fully dynamical model rather than the simple, empirical scheme used in System 4. There are also improvements in 2 m temperature skill in the vicinity of the Arctic sea-ice edge. Cold temperature biases in the troposphere improve, but increase at the tropopause. Biases in the extratropical jets are larger than in System 4: extratropical jets are too strong, and displaced northwards in JJA. In summary, development and added complexity since System 4 has ensured that SEAS5 is a state-of-The-Art seasonal forecast system which continues to display a particular strength in the El Niño Southern Oscillation (ENSO) prediction.

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An adaptation of the CO2 slicing technique for the Infrared Atmospheric Sounding Interferometer to obtain the height of tropospheric volcanic ash clouds

Copernicus Publications (2019) 1-48

Authors:

Isabelle A Taylor, Elisa Carboni, Lucy J Ventress, Tamsin A Mather, Roy G Grainger

Towards more representative gridded satellite products

IEEE Geoscience and Remote Sensing Letters IEEE 16:5 (2018) 672-676

Authors:

Adam Povey, Roy Grainger

Abstract:

The most widely used satellite products are averages of data onto a regular spatiotemporal grid, known as Level 3 data. Some atmospheric variables can vary rapidly in response to changing conditions. Over the scales of Level 3 averaging, the combination of observations across different conditions may result in data that is not normally distributed, such that a simple mean is not representative. The problem is illustrated by the distribution of aerosol optical depth from different sensors and algorithms. A simple statistical technique is proposed to better convey the diversity of satellite observations to users whereby a multimodal log-normal distribution is fit to the distribution of data observed within each grid cell. Allowing multiple modes within each cell is shown to improve the agreement between satellite products by highlighting regions of significant variability and isolating systematic differences between instruments.