Isentropic, diabatic, and sedimentary transport of Mount Pinatubo aerosol

Journal of Geophysical Research Atmospheres 104:D4 (1999) 4051-4063

Authors:

HL Rogers, WA Norton, A Lambert, RG Grainger

Abstract:

Observations of Mount Pinatubo aerosol as measured by the ISAMS instrument on UARS are presented for December 1991. These observations show a tropical reservoir of high aerosol with steep gradients across the subtropics. On the 450 K isentrope there is a ring of high aerosol in midlatitudes which is separated from the tropical reservoir by an approximately zonal band of lower aerosol values. The ISAMS aerosol data are compared with output from the off-line three-dimensional transport model SLIMCAT. Integrations are performed with isentropic transport only, diabatic transport only, isentropic and diabatic transport, and isentropic, diabatic and sedimentary transport of aerosol. Integrations using winds and temperatures from UKMO and ECMWF are compared. It is shown that even in the lower stratosphere, cross-isentropic transport over the timescale of a month can have a significant effect on the distribution of aerosol. The SLIMCAT integrations with isentropic transport only do not form a ring of high aerosol in midlatitudes on the 450 K isentrope. Inclusion of diabatic transport in the SLIMCAT integration shows that this ring forms from diabatic descent of air containing higher aerosol concentrations from aloft. Isentropic transport of high-aerosol air from the tropics into midlatitudes on the 500 K isentrope, followed by diabatic descent, further increases the values in the midlatitude ring on the 450 K isentrope. Inclusion of the sedimentation of aerosol in SLIMCAT integrations significantly offsets the diabatic ascent in the tropics. The SLIMCAT integrations, particularly those run using UKMO analyses, produce too much transport of midlatitude air into the tropics. The implications for accurate modeling of the tropical reservoir are discussed. Copyright 1999 by the American Geophysical Union.

Isentropic, diabatic, and sedimentary transport of Mount Pinatubo aerosol

J GEOPHYS RES-ATMOS 104 (1999) 4051–4063-4051–4063

Authors:

HL Rogers, WA Norton, A Lambert, RG Grainger

Abstract:

Observations of Mount Pinatubo aerosol as measured by the ISAMS instrument on UARS are presented for December 1991. These observations show a tropical reservoir of high aerosol with steep gradients across the subtropics. On the 450 K isentrope there is a ring of high aerosol in midlatitudes which is separated from the tropical reservoir by an approximately zonal band of lower aerosol values. The ISAMS aerosol data are compared with output from the off-line three-dimensional transport model SLIMCAT. Integrations are performed with isentropic transport only, diabatic transport only, isentropic and diabatic transport, and isentropic, diabatic and sedimentary transport of aerosol. Integrations using winds and temperatures from UKMO and ECMWF are compared. It is shown that even in the lower stratosphere, cross-isentropic transport over the timescale of a month can have a significant effect on the distribution of aerosol. The SLIMCAT integrations with isentropic transport only do not form a ring of high aerosol in midlatitudes on the 450 K isentrope. Inclusion of diabatic transport in the SLIMCAT integration shows that this ring forms from diabatic descent of air containing higher aerosol concentrations from aloft. Isentropic transport of high-aerosol air from the tropics into midlatitudes on the 500 K isentrope, followed by diabatic descent, further increases the values in the midlatitude ring on the 450 K isentrope. Inclusion of the sedimentation of aerosol in SLIMCAT integrations significantly offsets the diabatic ascent in the tropics. The SLIMCAT integrations, particularly those run using UKMO analyses, produce too much transport of midlatitude air into the tropics. The implications for accurate modeling of the tropical reservoir are discussed.

Infrared and visible Fourier-transform spectra of sulfuric-acid-water aerosols at 230 and 294 K

APPLIED OPTICS 38:30 (1999) 6408-6420

Authors:

AE Heathfield, DA Newnham, J Ballard, RG Grainger, A Lambert

A three-dimensional model simulation of the impact of Mt. Pinatubo aerosol on the Antarctic ozone hole

Quarterly Journal of the Royal Meteorological Society Wiley 124:549 (1998) 1527-1558

Authors:

JR KNIGHT, JOHN AUSTIN, RG GRAINGER, A LAMBERT

Radiative forcing from the 1991 Mount Pinatubo volcanic eruption

J GEOPHYS RES-ATMOS 103 (1998) 13837–13857-13837–13857

Authors:

GL Stenchikov, I Kirchner, A Robock, HF Graf, JC Antuna, RG Grainger, A Lambert, L Thomason

Abstract:

Volcanic sulfate aerosols in the stratosphere produce significant long-term solar and infrared radiative perturbations in the Earth’s atmosphere and at the surface, which cause a response of the climate system. Here we study the fundamental process of the development of this volcanic radiative forcing, focusing on the eruption of Mount Pinatubo in the Philippines on June 15, 1991. We develop a spectral-, space-, and time-dependent set of aerosol parameters for 2 years after the Pinatubo eruption using a combination of SAGE II aerosol extinctions and UARS-retrieved effective radii, supported by SAM II, AVHRR, lidar and balloon observations. Using these data, we calculate the aerosol radiative forcing with the ECHAM4 general circulation model (GCM) for cases with climatological and observed sea surface temperature (SST), as well as with and without climate response. We find that the aerosol radiative forcing is not sensitive to the climate variations caused by SST or the atmospheric response to the aerosols, except in regions with varying dense cloudiness. The solar forcing in the near infrared contributes substantially to the total stratospheric heating. A complete formulation of radiative forcing should include not only changes of net fluxes at the tropopause but also the vertical distribution of atmospheric heating rates and the change of downward thermal and net solar radiative fluxes at the surface. These forcing and aerosol data are available for GCM experiments with any spatial and spectral resolution.