Global atmospheric chemistry from satellites: Results from UARS/ISAMS

FARADAY DISCUSS (1995) 353-369

Authors:

FW Taylor, CD Rodgers, JJ Remedios, RG Grainger, A Lambert, M LopezValverde, M GossCustard, J Reburn

Abstract:

Satellites are a relatively new tool for investigating atmospheric chemical processes and their products. The precision and, in particular, the space and time coverage, now being achieved is immensely useful, and often essential, where global-scale phenomena like the variability of the stratospheric ozone layer are under study. The IR remote-sensing method using pressure modulator radiometry has recently been extended to the mapping of trace species. The technique is described, and its capabilities demonstrated with some selected new results from the improved stratospheric and mesopheric sounder (ISAMS) on the upper atmosphere research satellite (UARS). ISAMS was designed to study nitrogen-catalysed ozone chemistry, plus transport and other processes involving water vapour, methane and carbon monoxide, in the middle atmosphere. Its primary products are fields of temperature and composition, including all of the important members of the active nitrogen family, water, methane, carbon monoxide, ozone, aerosols and ice clouds. In the new data, all of these show large variations with time, height and latitude. The results have not yet been fully analysed, but early indications are that they confirm some models based on theoretical predictions and earlier, more limited, data, while in other cases they show that the situation is more complex than had been assumed. Sophisticated studies of the radiative-chemical-dynamical system in the stratosphere using satellite data and computer models are now in progress. In the future, even more advanced sensors now being built will obtain improved spatial resolution in the stratosphere, and map the global budgets of tropospheric trace gases as well.

Global atmospheric chemistry from satellites: Results from UARS/ISAMS

FARADAY DISCUSS (1995) 353–369-353–369

Authors:

FW Taylor, CD Rodgers, JJ Remedios, RG Grainger, A Lambert, M LopezValverde, M GossCustard, J Reburn

Abstract:

Satellites are a relatively new tool for investigating atmospheric chemical processes and their products. The precision and, in particular, the space and time coverage, now being achieved is immensely useful, and often essential, where global-scale phenomena like the variability of the stratospheric ozone layer are under study. The IR remote-sensing method using pressure modulator radiometry has recently been extended to the mapping of trace species. The technique is described, and its capabilities demonstrated with some selected new results from the improved stratospheric and mesopheric sounder (ISAMS) on the upper atmosphere research satellite (UARS). ISAMS was designed to study nitrogen-catalysed ozone chemistry, plus transport and other processes involving water vapour, methane and carbon monoxide, in the middle atmosphere. Its primary products are fields of temperature and composition, including all of the important members of the active nitrogen family, water, methane, carbon monoxide, ozone, aerosols and ice clouds. In the new data, all of these show large variations with time, height and latitude. The results have not yet been fully analysed, but early indications are that they confirm some models based on theoretical predictions and earlier, more limited, data, while in other cases they show that the situation is more complex than had been assumed. Sophisticated studies of the radiative-chemical-dynamical system in the stratosphere using satellite data and computer models are now in progress. In the future, even more advanced sensors now being built will obtain improved spatial resolution in the stratosphere, and map the global budgets of tropospheric trace gases as well.

STRATOSPHERIC AEROSOL EFFECTIVE RADIUS, SURFACE-AREA AND VOLUME ESTIMATED FROM INFRARED MEASUREMENTS

JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 100:D8 (1995) 16507-16518

Authors:

RG GRAINGER, A LAMBERT, CD RODGERS, FW TAYLOR, T DESHLER

PROPERTIES OF NORTHERN-HEMISPHERE POLAR STRATOSPHERIC CLOUDS AND VOLCANIC AEROSOL IN 1991/92 FROM UARS ISAMS SATELLITE MEASUREMENTS

J ATMOS SCI 51 (1994) 3019–3026-3019–3026

Authors:

FW TAYLOR, A LAMBERT, RG GRAINGER, CD RODGERS, JJ REMEDIOS

Abstract:

Observations of polar stratospheric clouds by the Improved Stratospheric and Mesospheric Sounder (ISAMS) experiment on the Upper Atmospheric Research Satellite (UARS) have revealed new details of their global properties and behavior. These include the vertical and horizontal spatial distributions of Arctic and Antarctic polar stratospheric clouds (PSCs) as a function of time and air temperature, their optical thicknesses and estimated densities, their spectral properties, and their inferred composition. In particular, ISAMS spectral data allows different PSC types to be distinguished from each other and from volcanic aerosol by their compositional differences. Northern PSCs during the 1991/92 season are found to be more ephemeral and more compact than reported in previous years and to differ markedly in scale from those in Southern Hemisphere, which cause the Antarctic ozone hole by activating stratospheric chlorine chemistry. There were only two episodes of dense PSC formation in the 1991/92 northern winter, one of which took place in sunlight. The latter correlates well with UARS/Microwave Limb Sounder observations of enhanced chlorine monoxide, but substantial amounts of chlorine monoxide were also reported at times and places with at most very minor PSC activity.

PROPERTIES OF NORTHERN-HEMISPHERE POLAR STRATOSPHERIC CLOUDS AND VOLCANIC AEROSOL IN 1991/92 FROM UARS ISAMS SATELLITE MEASUREMENTS

JOURNAL OF THE ATMOSPHERIC SCIENCES 51:20 (1994) 3019-3026

Authors:

FW TAYLOR, A LAMBERT, RG GRAINGER, CD RODGERS, JJ REMEDIOS