Single crystal growth from separated educts and its application to lithium transition-metal oxides

(2016)

Authors:

F Freund, SC Williams, RD Johnson, R Coldea, P Gegenwart, A Jesche

Incommensurate Counterrotating Magnetic Order Stabilized by Kitaev Interactions in the Layered Honeycomb ${\alpha}$-Li$_2$IrO$_3$

(2016)

Authors:

SC Williams, RD Johnson, F Freund, Sungkyun Choi, A Jesche, I Kimchi, S Manni, A Bombardi, P Manuel, P Gegenwart, R Coldea

Incommensurate counterrotating magnetic order stabilized by Kitaev interactions in the layered honeycomb alpha-Li2IrO3

University of Oxford (2016)

Authors:

Stephanie Williams, Roger Johnson, Radu Coldea, Itamar Kimchi

Abstract:

This dataset contains plain text files containing the data presented in Figures 1, 2, 3, and 4 of the corresponding manuscript published in Physical Review B. See readme.txt.

Single crystal growth from separated educts and its application to lithium transition-metal oxides: Data archive

University of Oxford (2016)

Authors:

Stephanie Williams, Roger Johnson, Radu Coldea

Abstract:

the deposited package contains single-crystal x-ray diffraction data from which the crystal structure of alpha-Li2IrO3 was refined.

Spin dynamics of counterrotating Kitaev spirals via duality

Physical Review B American Physical Society 94:20 (2016) 201110(R)

Authors:

I Kimchi, Radu Coldea

Abstract:

Incommensurate spiral order is a common occurrence in frustrated magnetic insulators. Typically, all magnetic moments rotate uniformly, through the same wavevector. However the honeycomb iridates family Li2IrO3 shows an incommensurate order where spirals on neighboring sublattices are counter-rotating, giving each moment a different local environment. Theoretically describing its spin dynamics has remained a challenge: the Kitaev interactions proposed to stabilize this state, which arise from strong spin-orbit effects, induce magnon umklapp scattering processes in spin-wave theory. Here we propose an approach via a (Klein) duality transformation into a conventional spiral of a frustrated Heisenberg model, allowing a direct derivation of the dynamical structure factor. We analyze both Kitaev and Dzyaloshinskii-Moriya based models, both of which can stabilize counterrotating spirals, but with different spin dynamics, and we propose experimental tests to identify the origin of counterrotation.