Professor Stephen Blundell

Abstract:

We had observed earlier that in the quaternary borocarbide magnetic superconductor TmNi2B2C (T-c = 11K, T-N = 1.5 K) quasistatic magnetic correlations persist well above TN (up to similar to 20 K), which is rather unusual. To further probe the nature of its spin state, we used magnetically oriented powder samples of TmNi2B2C and the mu-SR technique. We observe that the quasistatic internal held has a well defined direction. The spontaneous muon precession signal has three times the amplitude when the c-axis alignment is perpendicular to the initial muon beam polarization than when parallel. The transverse configuration enhances the oscillatory signal. This has enabled us to show that the quasistatic magnetic correlations persist even up to 50 K. Furthermore, we find a peak around 7 G in the field dependence of the longitudinal relaxation, which we attribute to the presence of a level crossing resonance arising from quadrupole levels of the boron nuclei. (C) 1999 Published by Elsevier Science B.V. All rights reserved.

Abstract:

Recent results of magnetization, magnetic susceptibility and muon spin rotation/relaxation (mu SR) measurements of some organic neutral radicals based on aminoxyl and their anion radical complexes with all;ali and transition metal cations are reported. Ferromagnetic intermolecular interactions, coexistent with antiferromagnetic ones, in several carboxyaryl nitronyl nitroxide radicals are affected by inserting alkali metal ions, while the incorporation of transition metal ions result in complex behavior suggesting in part ferromagnetic interactions. Temperature dependence of spontaneous magnetization of TANOL suberate in the ordered state, obtained through the results of mu SR measurements, is characteristic of a two-dimensional magnetic lattice, consistent with that of magnetic susceptibility above the ordering temperature.

Abstract:

Fermi-surface traversal resonance (FTR) is caused by the periodic motion of carriers in a magnetic field across open sections of Fermi surface (FS). Owing to the warping of the FS, the real space velocities of the carriers oscillate, generating resonances in the high frequency conductivity which may be described by a semiclassical model. A rectangular resonant cavity, oscillating at 70 GHz, which can rotate in the external magnetic field, has been used to confirm the existence of the effect in the organic metal alpha-(BEDT-TTF)(2)KHg(SCN)(4). The data contain a great deal of information about the FS, including the direction and anharmonicity of warping components. A quantum mechanical model is presented which predicts all of the features of FTR appearing in the semiclassical model. This confirms that FTR is a fundamental property of few-dimensional systems, existing under a very wide range of conditions.

Abstract:

Recent results of magnetization, magnetic susceptibility and muon spin rotation/relaxation (mu SR) measurements of some organic neutral radicals based on aminoxyl and their anion radical complexes with alkali and transition metal cations are reported. Ferromagnetic intermolecular interactions, coexistent with antiferromagnetic ones, in several carboxyaryl nitronyl nitroxide radicals are affected by inserting alkali metal ions, while the incorporation of transition metal ions result in complex behavior suggesting in part ferromagnetic interactions. Temperature dependence of spontaneous magnetization of TANOL suberate in the ordered state, obtained through the results of ASR measurements, is characteristic of a two-dimensional magnetic lattice, consistent with that of magnetic susceptibility above the ordering temperature.