Skip to main content
Home
Department Of Physics text logo
  • Research
    • Our research
    • Our research groups
    • Our research in action
    • Research funding support
    • Summer internships for undergraduates
  • Study
    • Undergraduates
    • Postgraduates
  • Engage
    • For alumni
    • For business
    • For schools
    • For the public
Menu
Crystal structure inside calcium fluoride with an implanted muon
Credit: SJB

Professor Stephen Blundell

Professor of Physics

Research theme

  • Quantum materials

Sub department

  • Condensed Matter Physics

Research groups

  • Muons and magnets
Stephen.Blundell@physics.ox.ac.uk
Telephone: 01865 (2)72347
Clarendon Laboratory, room 108
  • About
  • Books
  • Teaching
  • Research
  • Publications

Electronic structure calculations for muon spectroscopy

Electronic Structure IOP Publishing (2025)

Authors:

Stephen Blundell, Miki Bonacci, Pietro Bonfà, Roberto De Renzi, Benjamin Huddart, Tom Lancaster, Leandro Miguel Liborio, Ifeanyi John Onuorah, Giovanni Pizzi, Francis Pratt, John Wilkinson

Abstract:

Abstract Muon spectroscopy has become a leading tool for the investigation of local magnetic fields in condensed matter physics, finding applications in the study of superconductivity, magnetism, ionic diffussion in battery materials, and numerous other fields. Though the muon yields quantitative information about the material, this can only be fully interpreted if the nature of the muon site and its stability is fully understood. Electronic structure calculations are of paramount importance for providing this understanding, particularly through a group of techniques that has become known as DFT+µ, density functional theory including the presence of the implanted muon. We describe how these electronic structure calculations can be used to underpin muon spectroscopy, and some examples of the science that follows from this, as well as some of the available software tools that are currently being developed.
More details from the publisher

Muon Studies of Superconductors

Annual Review of Condensed Matter Physics Annual Reviews 16:1 (2025) 367-385
More details from the publisher

Spiral spin liquid noise.

Proceedings of the National Academy of Sciences of the United States of America 122:12 (2025) e2422498122

Authors:

Hiroto Takahashi, Chun-Chih Hsu, Fabian Jerzembeck, Jack Murphy, Jonathan Ward, Jack D Enright, Jan Knapp, Pascal Puphal, Masahiko Isobe, Yosuke Matsumoto, Hidenori Takagi, JC Séamus Davis, Stephen J Blundell

Abstract:

An emerging concept for identification of different types of spin liquids [C. Broholm et al., Science 367, eaay0668 (2020)] is through the use of spontaneous spin noise [S. Chatterjee, J. F. Rodriguez-Nieva, E. Demler, Phys. Rev. B 99, 104425 (2019)]. Here, we develop spin noise spectroscopy for spin liquid studies by considering Ca10Cr7O28, a material hypothesized to be either a quantum or a spiral spin liquid (SSL). By enhancing techniques introduced for magnetic monopole noise studies [R. Dusad et al., Nature 571, 234-239 (2019)], we measure the time and temperature dependence of spontaneous flux [Formula: see text] and thus magnetization [Formula: see text] of Ca10Cr7O28 samples. The resulting power spectral density of magnetization noise [Formula: see text] reveals intense spin fluctuations with [Formula: see text] and [Formula: see text]. Both the variance [Formula: see text] and the correlation function [Formula: see text] of this spin noise undergo crossovers at a temperature [Formula: see text]. While predictions for quantum spin liquids are inconsistent with this phenomenology, those from Monte-Carlo simulations of a two-dimensional (2D) SSL state in Ca10Cr7O28 yield overall quantitative correspondence with the measured frequency and temperature dependences of [Formula: see text], and [Formula: see text], thus indicating that Ca10Cr7O28 is an SSL.
More details from the publisher
More details
More details

Field-orientation-dependent magnetic phases in GdRu2Si2 probed with muon-spin spectroscopy

Physical Review B American Physical Society (APS) 111:5 (2025) 54440

Authors:

Bm Huddart, A Hernández-Melián, Gda Wood, Da Mayoh, M Gomilšek, Z Guguchia, C Wang, Tj Hicken, Sj Blundell, G Balakrishnan, T Lancaster

Abstract:

<jats:p>Centrosymmetric <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"><a:mrow><a:msub><a:mi>GdRu</a:mi><a:mn>2</a:mn></a:msub><a:msub><a:mi>Si</a:mi><a:mn>2</a:mn></a:msub></a:mrow></a:math> exhibits a variety of multi-<b:math xmlns:b="http://www.w3.org/1998/Math/MathML"><b:mrow><b:mi>Q</b:mi></b:mrow></b:math> magnetic states as a function of temperature and applied magnetic field, including a square skyrmion-lattice phase. The material's behavior is strongly dependent on the direction of the applied field, with different phase diagrams resulting for fields applied parallel or perpendicular to the crystallographic <c:math xmlns:c="http://www.w3.org/1998/Math/MathML"><c:mi>c</c:mi></c:math> axis. Here, we present the results of muon-spin relaxation (<d:math xmlns:d="http://www.w3.org/1998/Math/MathML"><d:mrow><d:msup><d:mi>μ</d:mi><d:mo>+</d:mo></d:msup><d:mi>SR</d:mi></d:mrow></d:math>) measurements on single crystals of <e:math xmlns:e="http://www.w3.org/1998/Math/MathML"><e:mrow><e:msub><e:mi>GdRu</e:mi><e:mn>2</e:mn></e:msub><e:msub><e:mi>Si</e:mi><e:mn>2</e:mn></e:msub></e:mrow></e:math>. Our analysis is based on the computation of muon stopping sites and consideration of quantum zero-point motion effects of muons, allowing direct comparison with the underlying spin textures in the material. The muon site is confirmed experimentally, using angle-dependent measurements of the muon Knight shift. Using transverse-field <f:math xmlns:f="http://www.w3.org/1998/Math/MathML"><f:msup><f:mi>μ</f:mi><f:mo>+</f:mo></f:msup><f:mi>SR</f:mi></f:math> with fields applied along either the [001] or [100] crystallographic directions, we distinguish between the magnetic phases in this system via their distinct muon response, providing additional evidence for the skyrmion and meron-lattice phases, while also suggesting the existence of RKKY-driven muon hyperfine coupling. Zero-field <g:math xmlns:g="http://www.w3.org/1998/Math/MathML"><g:mrow><g:msup><g:mi>μ</g:mi><g:mo>+</g:mo></g:msup><g:mi>SR</g:mi></g:mrow></g:math> provides clear evidence for a transition between two distinct magnetically ordered phases at 39 K.</jats:p> <jats:sec> <jats:title/> <jats:supplementary-material> <jats:permissions> <jats:copyright-statement>Published by the American Physical Society</jats:copyright-statement> <jats:copyright-year>2025</jats:copyright-year> </jats:permissions> </jats:supplementary-material> </jats:sec>
More details from the publisher
More details

Coexistence of Kondo coherence and localized magnetic moments in the normal state of molten salt-flux grown UTe2

Physical Review B American Physical Society (APS) 111:1 (2025) 014513

Authors:

N Azari, M Yakovlev, SR Dunsiger, OP Uzoh, E Mun, BM Huddart, SJ Blundell, MM Bordelon, SM Thomas, JD Thompson, PFS Rosa, JE Sonier
More details from the publisher
More details

Pagination

  • Current page 1
  • Page 2
  • Page 3
  • Page 4
  • Page 5
  • Page 6
  • Page 7
  • Page 8
  • Page 9
  • …
  • Next page Next
  • Last page Last

Footer Menu

  • Contact us
  • Giving to the Dept of Physics
  • Work with us
  • Media

User account menu

  • Log in

Follow us

FIND US

Clarendon Laboratory,

Parks Road,

Oxford,

OX1 3PU

CONTACT US

Tel: +44(0)1865272200

University of Oxfrod logo Department Of Physics text logo
IOP Juno Champion logo Athena Swan Silver Award logo

© University of Oxford - Department of Physics

Cookies | Privacy policy | Accessibility statement

Built by: Versantus

  • Home
  • Research
  • Study
  • Engage
  • Our people
  • News & Comment
  • Events
  • Our facilities & services
  • About us
  • Current students
  • Staff intranet