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CMP
Credit: Jack Hobhouse

Dr Dharmalingam Prabhakaran

Researcher

Research theme

  • Quantum materials

Sub department

  • Condensed Matter Physics

Research groups

  • Synthesis and crystal growth
dharmalingam.prabhakaran@physics.ox.ac.uk
Telephone: 01865 (2)72270,01865 (2)72351,01865 (2)72341
Clarendon Laboratory, room 177,377,373
  • About
  • Publications

Restoration of the third law in spin ice thin films

Nature Communications Springer Nature 5 (2014) 3439

Authors:

L Bovo, X Moya, D Prabhakaran, YA Soh, Andrew Boothroyd, ND Mathur, G Aeppli, ST Bramwell

Abstract:

A characteristic feature of spin ice is its apparent violation of the third law of thermodynamics. This leads to a number of interesting properties including the emergence of an effective vacuum for magnetic monopoles and their currents – magnetricity. Here we add a new dimension to the experimental study of spin ice by fabricating thin epitaxial films of Dy2Ti2O7, varying between 5 and 60 monolayers on an inert substrate. The films show the distinctive characteristics of spin ice at temperatures >2 K, but at lower temperature we find evidence of a zero entropy state. This restoration of the third law in spin ice thin films is consistent with a predicted strain-induced ordering of a very unusual type, previously discussed for analogous electrical systems. Our results show how the physics of frustrated pyrochlore magnets such as spin ice may be significantly modified in thin-film samples.
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Stripe disorder and dynamics in the hole-doped antiferromagnetic insulator la 5 / 3 Sr 1 / 3 CoO 4

Physical Review B - Condensed Matter and Materials Physics 89:2 (2014)

Authors:

T Lancaster, SR Giblin, G Allodi, S Bordignon, M Mazzani, R De Renzi, PG Freeman, PJ Baker, FL Pratt, P Babkevich, SJ Blundell, AT Boothroyd, JS Möller, D Prabhakaran

Abstract:

We investigate the magnetic ordering and dynamics of the stripe phase of La5/3Sr1/3CoO4, a material shown to have an hourglass magnetic excitation spectrum. A combination of muon-spin relaxation, nuclear magnetic resonance, and magnetic susceptibility measurements strongly suggest that the physics is determined by a partially disordered configuration of charge and spin stripes whose frustrated magnetic degrees of freedom are dynamic at high temperature and which undergo an ordering transition around 35 K with coexisting dynamics that freeze out in a glassy manner as the temperature is further reduced. © 2014 American Physical Society.
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A stable three-dimensional topological Dirac semimetal Cd3 As2

Nature Materials 13:7 (2014) 677-681

Authors:

ZK Liu, J Jiang, B Zhou, ZJ Wang, Y Zhang, HM Weng, D Prabhakaran, SK Mo, H Peng, P Dudin, T Kim, M Hoesch, Z Fang, X Dai, ZX Shen, DL Feng, Z Hussain, YL Chen

Abstract:

Three-dimensional (3D) topological Dirac semimetals (TDSs) are a recently proposed state of quantum matter 1-6that have attracted increasing attention in physics and materials science. A 3D TDS is not only a bulk analogue of graphene; it also exhibits non-trivial topology in its electronic structure that shares similarities with topological insulators. Moreover, a TDS can potentially be driven into other exotic phases (such as Weyl semimetals, axion insulators and topological superconductors), making it a unique parent compound for the study of these states and the phase transitions between them. Here, by performing angle-resolved photoemission spectroscopy, we directly observe a pair of 3D Dirac fermions in Cd3 As2, proving that it is a model 3D TDS. Compared with other 3D TDSs, for example, β-cristobalite BiO2 (ref.) and Na 3 Bi (refs,), Cd3 As2 is stable and has much higher Fermi velocities. Furthermore, by in situ doping we have been able to tune its Fermi energy, making it a flexible platform for exploring exotic physical phenomena. © 2014 Macmillan Publishers Limited. All rights reserved.
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Discovery of a three-dimensional topological dirac semimetal, Na 3Bi

Science 343:6173 (2014) 864-867

Authors:

ZK Liu, B Zhou, Y Zhang, ZJ Wang, HM Weng, D Prabhakaran, SK Mo, ZX Shen, Z Fang, X Dai, Z Hussain, YL Chen

Abstract:

Three-dimensional (3D) topological Dirac semimetals (TDSs) represent an unusual state of quantum matter that can be viewed as "3D graphene." In contrast to 2D Dirac fermions in graphene or on the surface of 3D topological insulators, TDSs possess 3D Dirac fermions in the bulk. By investigating the electronic structure of Na3Bi with angle-resolved photoemission spectroscopy, we detected 3D Dirac fermions with linear dispersions along all momentum directions. Furthermore, we demonstrated the robustness of 3D Dirac fermions in Na3Bi against in situ surface doping. Our results establish Na3Bi as a model system for 3D TDSs, which can serve as an ideal platform for the systematic study of quantum phase transitions between rich topological quantum states.
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Far-from-equilibrium monopole dynamics in spin ice

Nature Physics 10:2 (2014) 135-139

Authors:

C Paulsen, MJ Jackson, E Lhotel, B Canals, D Prabhakaran, K Matsuhira, SR Giblin, ST Bramwell

Abstract:

Condensed matter in the low-temperature limit reveals exotic physics associated with unusual orders and excitations, with examples ranging from helium superfluidity to magnetic monopoles in spin ice. The far-from-equilibrium physics of such low-temperature states may be even more exotic, yet to access it in the laboratory remains a challenge. Here we demonstrate a simple and robust technique - the 'magnetothermal avalanche quench' - and its use in the controlled creation of non-equilibrium populations of magnetic monopoles in spin ice at millikelvin temperatures. These populations are found to exhibit spontaneous dynamical effects that typify far-from-equilibrium systems and yet are captured by simple models. Our method thus opens new directions in the study of far-from-equilibrium states in spin ice and other exotic magnets. © 2014 Macmillan Publishers Limited.
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