What controls the vertical distribution of aerosol? Relationships between process sensitivity in HadGEM3–UKCA and inter-model variation from AeroCom Phase II

Atmospheric Chemistry and Physics 16 (2016) 2221-2241

Authors:

Z Kipling, P Stier, CE Johnson, GW Mann, N Bellouin, SE Bauer, T Bergman, M Chin, T Diehl, SJ Ghan, T Iversen, A Kirkevåg, H Kokkola, X Liu, G Luo, T van Noije, KJ Pringle, K von Salzen, M Schulz, Ø Seland, RB Skeie, T Takemura, K Tsigaridis, K Zhang

The importance of temporal collocation for the evaluation of aerosol models with observations

Atmospheric Chemistry and Physics European Geosciences Union 16:2 (2016) 1065-1079

Authors:

Nick AJ Schutgens, Dan G Partridge, Philip Stier

Abstract:

It is often implicitly assumed that over suitably long periods the mean of observations and models should be comparable, even if they have different temporal sampling. We assess the errors incurred due to ignoring temporal sampling and show that they are of similar magnitude as (but smaller than) actual model errors (20–60 %).

Using temporal sampling from remote-sensing data sets, the satellite imager MODIS (MODerate resolution Imaging Spectroradiometer) and the ground-based sun photometer network AERONET (AErosol Robotic NETwork), and three different global aerosol models, we compare annual and monthly averages of full model data to sampled model data. Our results show that sampling errors as large as 100 % in AOT (aerosol optical thickness), 0.4 in AE (Ångström Exponent) and 0.05 in SSA (single scattering albedo) are possible. Even in daily averages, sampling errors can be significant. Moreover these sampling errors are often correlated over long distances giving rise to artificial contrasts between pristine and polluted events and regions. Additionally, we provide evidence that suggests that models will underestimate these errors. To prevent sampling errors, model data should be temporally collocated to the observations before any analysis is made.

We also discuss how this work has consequences for in situ measurements (e.g. aircraft campaigns or surface measurements) in model evaluation.

Although this study is framed in the context of model evaluation, it has a clear and direct relevance to climatologies derived from observational data sets.

Will a perfect model agree with perfect observations? The impact of spatial sampling

Copernicus Publications (2016)

Authors:

NAJ Schutgens, E Gryspeerdt, N Weigum, S Tsyro, D Goto, M Schulz, P Stier

Limitations of passive satellite remote sensing to constrain global cloud condensation nuclei

Atmospheric Chemistry and Physics European Geosciences Union 15:22 (2015) 32607-32637

Abstract:

Aerosol–cloud interactions are considered a key uncertainty in our understanding of climate change (Boucher et al., 2013). Knowledge of the global abundance of aerosols suitable to act as cloud condensation nuclei (CCN) is fundamental to determine the strength of the anthropogenic climate perturbation. Direct measurements are limited and sample only a very small fraction of the globe so that remote sensing from satellites and ground based instruments is widely used as a proxy for cloud condensation nuclei (Nakajima et al., 2001; Andreae, 2009; Clarke and Kapustin, 2010; Boucher et al., 2013). However, the underlying assumptions cannot be robustly tested with the small number of measurements available so that no reliable global estimate of cloud condensation nuclei exists. This study overcomes this limitation using a fully self-consistent global model (ECHAM-HAM) of aerosol radiative properties and cloud condensation nuclei. An analysis of the correlation of simulated aerosol radiative properties and cloud condensation nuclei reveals that common assumptions about their relationships are violated for a significant fraction of the globe: 71 % of the area of the globe shows correlation coefficients between CCN0.2% at cloud base and aerosol optical depth (AOD) below 0.5, i.e. AOD variability explains only 25 % of the CCN variance. This has significant implications for satellite based studies of aerosol–cloud interactions. The findings also suggest that vertically resolved remote sensing techniques, such as satellite-based high spectral resolution lidars, have a large potential for global monitoring of cloud condensation nuclei.

Satellite observations of convection and their implications for parameterizations

Chapter in Parameterization of Atmospheric Convection, World Scientific Publishing 1 (2015) 47-58

Authors:

J Quaas, P Stier