Storing quantum information in chemically engineered nanoscale magnets

Journal of Materials Chemistry 19:12 (2009) 1754-1760

Authors:

A Ardavan, SJ Blundell

Abstract:

We review the implementation of quantum information processing using quantum spins and pulsed spin resonance techniques. Molecular magnets, nanoscale clusters of coupled transition metal ions, offer various potential advantages over other spin systems as the building blocks of a quantum computer. We describe the strategies which must be employed in order to implement quantum algorithms in such nanoscale magnets and explain why, when evaluating the suitability of any physical system for embodying a qubit, it is essential to determine the phase relaxation time appropriate for an individual molecular spin. Experiments utilising pulsed spin resonance techniques show that the phase relaxation times in at least some molecular magnets are long enough to permit multiple qubit operations to be performed. © The Royal Society of Chemistry 2009.

A new mechanism for generating broadband pulsar-like polarization

(2009)

Authors:

Houshang Ardavan, Arzhang Ardavan, Joseph Fasel, John Middleditch, Mario Perez, Andrea Schmidt, John Singleton

A bimetallic endohedral fullerene: PrSc@C80

Chemical Communications (2009) 4082-4084

Authors:

SR Plant, TC Ng, JH Warner, G Dantelle, A Ardavan, GAD Briggs, K Porfyrakis

Abstract:

The synthesis, isolation and characterization of a previously undiscovered bimetallic endohedral fullerene, PrSc@C80, are presented, and this may pave the way for a whole family of bimetallic endohedral fullerenes in useful quantities. © 2009 The Royal Society of Chemistry.

Acuminated fluorescence of Er3+ centres in endohedral fullerenes through the incarceration of a carbide cluster

CHEMICAL PHYSICS LETTERS 476:1-3 (2009) 41-45

Authors:

Simon R Plant, Geraldine Dantelle, Yasuhiro Ito, Tsz Cheong Ng, Arzhang Ardavan, Hisanori Shinohara, Robert A Taylor, G Andrew D Briggs, Kyriakos Porfyrakis

Clocking the Collapse of a Mott Gap

ULTRAFAST PHENOMENA XVI 92 (2009) 167-+

Authors:

S Wall, D Brida, HP Ehrke, A Ardavan, S Bonora, H Matsusaki, H Uemura, Y Takahashi, T Hasegawa, H Okamoto, G Cerullo, A Cavalleri