Dr Nick Bultinck

Abstract:

A striking series of experiments have observed superconductivity in Bernal-stacked bilayer graphene (BBG) when the energy bands are flattened by applying an electrical displacement field. Intriguingly, superconductivity manifests only at nonzero magnetic fields, or when spin-orbit coupling is induced in BBG by coupling to a substrate. We present detailed functional renormalization group and random-phase approximation calculations that provide a unified explanation for the superconducting mechanism in both cases. Both calculations yield a purely electronic 𝑝-wave instability of the Kohn-Luttinger type. The latter can be enhanced either by magnetic fields or Ising spin-orbit coupling, naturally explaining the behavior seen in experiments.

Abstract:

Recent scanning tunneling microscopy experiments in twisted bilayer [K. P. Nuckolls et al., Nature (London) 620, 525 (2023)] and trilayer [H. Kim et al., Nature (London) 623, 942 (2023)] graphene have revealed the ubiquity of Kekulé charge-density wave order in magic-angle graphene. Most samples are moderately strained and show “incommensurate Kekulé spiral” (IKS) order involving a graphene-scale charge density distortion uniaxially modulated on the scale of the moiré superlattice, in accord with theoretical predictions. However, ultralow strain bilayer samples instead show graphene-scale Kekulé charge order that is uniform on the moiré scale. This order, especially prominent near filling factor 𝜈=−2, is unanticipated by theory which predicts a time-reversal breaking Kekulé current order at low strain. We show that including the coupling of moiré electrons to graphene-scale optical zone-corner (ZC) phonons stabilizes a uniform Kekulé charge ordered state at |𝜈|=2 with a quantized topological (spin or anomalous Hall) response. Our work clarifies how this phonon-driven selection of electronic order emerges in the strong-coupling regime of moiré graphene.

Abstract:

Iron-chalcogenide superconductors display rich phenomena caused by orbital-dependent band shifts and electronic correlations. Additionally, they are potential candidates for topological superconductivity due to the band inversion between the Fe d bands and the chalcogen p_z band. Here we present a detailed study of the electronic structure of the nematic superconductors FeSe_1−xTe_x (0 < x < 0.4) using angle-resolved photoemission spectroscopy to understand the role of orbital-dependent band shifts, electronic correlations and the chalcogen band. We assess the changes in the effective masses using a three-band low energy model, and the band renormalization via comparison with DFT band structure calculations. The effective masses decrease for all three-hole bands inside the nematic phase, followed by a strong increase for the band with d_xy orbital character. Interestingly, this nearly-flat d_xy band becomes more correlated as it shifts towards the Fermi level with increasing Te concentrations and as the second superconducting dome emerges. Our findings suggests that the d_xy hole band, which is very sensitive to the chalcogen height, could be involved in promoting an additional pairing channel and increasing the density of states to stabilize the second superconducting dome in FeSe_1−xTe_x. This simultaneous shift of the d_xy hole band and enhanced superconductivity is in contrast with FeSe_1−xS_x.