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CMP
Credit: Jack Hobhouse

Dr Dharmalingam Prabhakaran

Researcher

Research theme

  • Quantum materials

Sub department

  • Condensed Matter Physics

Research groups

  • Synthesis and crystal growth
dharmalingam.prabhakaran@physics.ox.ac.uk
Telephone: 01865 (2)72270,01865 (2)72351,01865 (2)72341
Clarendon Laboratory, room 177,377,373
  • About
  • Publications

Critical behavior of the paramagnetic to antiferromagnetic transition in orthorhombic and hexagonal phases of RMnO 3 (R=Sm, Tb, Dy, Ho, Er, Tm, Yb, Lu, Y)

Physical Review B - Condensed Matter and Materials Physics 85:18 (2012)

Authors:

A Oleaga, A Salazar, D Prabhakaran, JG Cheng, JS Zhou

Abstract:

The critical behavior of the paramagnetic to antiferromagnetic transition in RMnO 3 (R = Sm, Tb, Dy, Ho, Er, Tm, Yb, Lu, Y) has been studied with an ac photopyroelectric calorimeter, which gives simultaneously the thermal diffusivity and specific heat as a function of temperature with high resolution around the Néel temperature. RMnO 3 (R = Sm, Tb, Dy) has an orthorhombic perovskite structure, whereas the other manganites are hexagonal, thus revealing a strong thermal anisotropy. SmMnO 3 with type-A antiferromagnetic ordering exhibits a 3D-XY critical behavior, which could be attributed to the peculiar site anisotropy of Sm3 + and the exchange interaction between Mn3 + and Sm3 + ions. The sinusoidal spin ordering in TbMnO 3 and DyMnO 3 can be phenomenologically described by the 3D-Heisenberg model. Finally, the hexagonal manganites RMnO 3 (R = Ho, Er, Tm, Yb, Lu, Y) are close to the 3D-Heisenberg universality class, ruling out the chiral models predicted by the renormalization group theory. © 2012 American Physical Society.
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Persistent dynamics in the S=1/2 quasi-one-dimensional chain compound Rb 4Cu(MoO 4) 3 probed with muon-spin relaxation

Physical Review B - Condensed Matter and Materials Physics 85:18 (2012)

Authors:

T Lancaster, PJ Baker, FL Pratt, SJ Blundell, W Hayes, D Prabhakaran

Abstract:

We report the results of muon-spin relaxation measurements on the low-dimensional antiferromagnet Rb 4Cu(MoO 4) 3. No long-range magnetic order is observed down to 50 mK implying a ratio T N/J<0.005 (where J is the principal exchange strength along the spin chains) and an effective ratio of interchain to intrachain exchange of |J ⊥/J|<2×10 -3, making the material an excellent realization of a one-dimensional quantum Heisenberg antiferromagnet. We probe the persistent spin excitations at low temperatures and find that ballistic spin transport dominates the excitations detected below 0.3 K. © 2012 American Physical Society.
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Electric field control of chiral magnetic domains in the high-temperature multiferroic CuO

Physical Review B - Condensed Matter and Materials Physics 85:13 (2012)

Authors:

P Babkevich, A Poole, RD Johnson, B Roessli, D Prabhakaran, AT Boothroyd

Abstract:

We have studied the high-temperature multiferroic cupric oxide using polarized neutron diffraction as a function of temperature and applied electric field. We find that the chiral domain population can be varied using an external electric field applied along the b axis. With the aid of representation analysis, we deduce the incommensurate magnetic structure in the multiferroic phase. We conclude that the origin of the magnetoelectric coupling is consistent with recently proposed models which are based on the inverse Dzyaloshinskii - Moriya interaction. © 2012 American Physical Society.
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Helical scattering signatures of strain and electronic textures in YbFe 2O 4 from three-dimensional reciprocal-space imaging

Physical Review B - Condensed Matter and Materials Physics 85:1 (2012)

Authors:

AJ Hearmon, D Prabhakaran, H Nowell, F Fabrizi, MJ Gutmann, PG Radaelli

Abstract:

The insulating ternary oxide YbFe 2O 4 displays an unusual frustration-driven incommensurate charge-ordering (CO) transition, linked to possible ferroelectricity. Based on high-resolution synchrotron data, we report a detailed structural model showing that the CO phase is an incommensurate charge-density wave and cannot be ferroelectric, since the electrical dipole moments are also incommensurately modulated. The change between continuous and "spotty" helices of scattering at the CO transition is attributed to three-dimensional fluctuations of the direction of the ordering wave vector. © 2012 American Physical Society.
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Evidence of magnetic correlations among the charge stripe electrons of charge-stripe ordered La2NiO4.11

Journal of Physics: Conference Series 340 (2012)

Authors:

PG Freeman, SM Hayden, RA Mole, M Enderle, D Prabhakaran, AT Boothroyd

Abstract:

The magnetic excitations of charge-stripe ordered La2NiO 4.11 where investigated using polarized- and unpolarized-neutron scattering to determine the magnetic excitations of the charge stripe electrons. We observed a magnetic excitation mode consistent with the gapped quasi-one-dimensional antiferromagnetic correlations of the charge stripe electrons previously observed in La2-xSrxNiO4 x = 1/3 and x = 0.275.
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