Effect of non-stoichiometry oxygen content on the magnetization of La 1.5 Sr 0.5 NiO 4+δ
Journal of Superconductivity and Novel Magnetism 24:3 (2011) 1149-1152
Abstract:
We report on magnetization measurements of La 1.5Sr 0.5NiO 4+δ for δ=0.01 and δ=-0.01. Zero field-cooled and field-cooled bulk magnetization measurements were performed parallel to the Ni-O planes of single crystals, and on a polycrystalline δ=0.01 sample. Striking differences in the magnetization curves are observed between the two doping levels that are identifiable in polycrystalline δ=0.01. The bulk magnetization differences indicate a crossover in the magnetic properties of La 2-x Sr x NiO 4+δ at half doping level, which can be used as a simple non-destructive way to determine whether La 1.5Sr 0.5NiO 4+δ is under or over half doping. © 2010 Springer Science+Business Media, LLC.Low-energy quasi-one-dimensional spin dynamics in charge-ordered La 2-x Srx NiO4
Physical Review B - Condensed Matter and Materials Physics 83:9 (2011)
Abstract:
The low-energy spin excitations of La2-xSrxNiO 4, x=0.275 and 1/3, have been investigated by unpolarized- and polarized-inelastic neutron scattering from single crystals. A pattern of magnetic diffuse scattering is observed in both compositions and is consistent with quasi-one-dimensional AFM spin correlations along the charge stripes. Analysis of the energy line shape for x=1/3 indicates that the diffuse scattering is inelastic with a characteristic energy of 1.40±0.07 meV. There is no discernible difference between the diffuse scattering from x=0.275 and x=1/3, suggesting that it is an intrinsic property of the charge stripes. © 2011 American Physical Society.Floating-zone growth of Na0.8-y Ay CoO2 (A=Ca, Sr) single crystals
Journal of Crystal Growth 318:1 (2011) 924-926
Abstract:
Single crystals of Na0.8-yAyCoO2 (A=Ca, Sr; y=0.10.3) have been grown using the optical floating-zone method for the first time. We have determined the optimum growth conditions to grow the highest quality single crystals. Columnar growth behavior has been observed for the higher doped samples. The magnetic and structural ordering temperatures of the doped samples were found to vary considerably. Crown Copyright © 2010 Published by Elsevier B.V. All rights reserved.Creation and measurement of long-lived magnetic monopole currents in spin ice
Nature Physics 7:3 (2011) 252-258
Abstract:
The recent discovery of 'magnetricity' in spin ice raises the question of whether long-lived currents of magnetic 'monopoles' can be created and manipulated by applying magnetic fields. Here we show that they can. By applying a magnetic-field pulse to a Dy 2 Ti 2 O 7 spin-ice crystal at 0.36 K, we create a relaxing magnetic current that lasts for several minutes. We measure the current by means of the electromotive force it induces in a solenoid coupled to a sensitive amplifier, and quantitatively describe it using a chemical kinetic model of point-like charges obeying the Onsager-Wien mechanism of carrier dissociation and recombination. We thus derive the microscopic parameters of monopole motion in spin ice and identify the distinct roles of free and bound magnetic charges. Our results illustrate a basic capacitor effect for magnetic charge and should pave the way for the design and realization of 'magnetronic' circuitry. © 2011 Macmillan Publishers Limited. All rights reserved.Bilayer manganites reveal polarons in the midst of a metallic breakdown
NATURE PHYSICS 7:12 (2011) 978-982