Gianluca Gregori

Abstract:

Complex multiscale flows associated with instabilities and turbulence are commonly induced under High Energy Density (HED) conditions, but accurate measurement of their transport properties has been challenging. X-ray Photon Correlation Spectroscopy (XPCS) with coherent X-ray sources can, in principle, probe material dynamics to infer transport properties using time autocorrelation of density fluctuations. Here we develop a theoretical framework for utilizing XPCS to study material diffusivity in multiscale flows. We extend single-scale shear flow theories to broadband flows using a multiscale analysis that captures shear and diffusion dynamics. Our theory is validated with simulated XPCS for Brownian particles advected in multiscale flows. We demonstrate the versatility of the method over several orders of magnitude in timescale using sequential-pulse XPCS, single-pulse X-ray Speckle Visibility Spectroscopy (XSVS), and double-pulse XSVS.

Abstract:

We extract electron transport properties from atomistic simulations of a two-component plasma by mapping the long-wavelength behavior to a two-fluid model. The mapping procedure is performed via Markov Chain Monte Carlo sampling over multiple spectra simultaneously. The free-electron dynamic structure factor and its properties have been investigated in the hydrodynamic formulation to justify its application to the long-wavelength behavior of warm dense matter. We have applied this method to warm dense hydrogen modeled with wave packet molecular dynamics and showed that the inferred electron transport properties are in agreement with a variety of reference calculations, except for the electron viscosity, where a substantive decrease is observed when compared to classical models.

Abstract:

<jats:p>We present new exclusion bounds obtained at the European X-Ray Free Electron Laser facility (EuXFEL) on axionlike particles in the mass range <a:math xmlns:a="http://www.w3.org/1998/Math/MathML" display="inline"><a:mrow><a:msup><a:mrow><a:mn>10</a:mn></a:mrow><a:mrow><a:mo>−</a:mo><a:mn>3</a:mn></a:mrow></a:msup><a:mtext> </a:mtext><a:mtext> </a:mtext><a:mrow><a:mi>eV</a:mi></a:mrow><a:mo>≲</a:mo><a:msub><a:mrow><a:mi>m</a:mi></a:mrow><a:mrow><a:mi>a</a:mi></a:mrow></a:msub><a:mo>≲</a:mo><a:msup><a:mrow><a:mn>10</a:mn></a:mrow><a:mrow><a:mn>4</a:mn></a:mrow></a:msup><a:mtext> </a:mtext><a:mtext> </a:mtext><a:mi>eV</a:mi></a:mrow></a:math>. Our experiment exploits the Primakoff effect via which photons can, in the presence of a strong external electric field, decay into axions, which then convert back into photons after passing through an opaque wall. While similar searches have been performed previously at a third-generation synchrotron [Yamaji , ], our work demonstrates improved sensitivity, exploiting the higher brightness of x-rays at EuXFEL.</jats:p> <jats:sec> <jats:title/> <jats:supplementary-material> <jats:permissions> <jats:copyright-statement>Published by the American Physical Society</jats:copyright-statement> <jats:copyright-year>2025</jats:copyright-year> </jats:permissions> </jats:supplementary-material> </jats:sec>

Abstract:

Recent cutting-edge experiments have provided in situ structure characterization and measurements of the pressure (P), density (¯ρ) and temperature (T) of shock compressed silicon in the 100 GPa range of pressures and up to ∼10,000K. We present first-principles calculations in this P, T, ρ¯ regime to reveal a plethora of novel liquid-liquid phase transitions (LPTs) identifiable via discontinuities in the pressure and the compressibility. Evidence for the presence of a highly-correlated liquid (CL) phase, as well as a normal-liquid (NL) phase at the LPTs is presented by a detailed study of one LPT. The LPTs make the interpretation of these experiments more challenging. The LPTs preserve the short-ranged ionic structure of the fluid by collective adjustments of many distant atoms when subject to compression and heating, with minimal change in the ion-ion pair-distribution functions, and in transport properties such as the electrical and thermal conductivities σ and κ. We match the experimental X-Ray Thomson scattering and X-ray diffraction data theoretically, and provide pressure isotherms, ionization data and compressibilities that support the above picture of liquid silicon as a highly complex LPT-driven “glassy” metallic liquid. These novel results are relevant to materials research, studies of planetary interiors, high-energy-density physics, and in laser-fusion studies.