Quantum interference between charge excitation paths in a solid-state Mott insulator
Nature Physics 7:2 (2011) 114-118
Abstract:
Competition between electron localization and delocalization in Mott insulators underpins the physics of strongly correlated electron systems. Photoexcitation, which redistributes charge, can control this many-body process on the ultrafast 1,2 timescale. So far, time-resolved studies have been carried out in solids in which other degrees of freedom, such as lattice, spin or orbital excitations 3-5 , dominate. However, the underlying quantum dynamics of bareg electronic excitations has remained out of reach. Quantum many-body dynamics are observed only in the controlled environment of optical lattices 6,7 where the dynamics are slower and lattice excitations are absent. By using nearly single-cycle near-infrared pulses, we have measured coherent electronic excitations in the organic salt ET-F 2 TCNQ, a prototypical one-dimensional Mott insulator. After photoexcitation, a new resonance appears, which oscillates at 25THz. Time-dependent simulations of the Mottg Hubbard Hamiltonian reproduce the oscillations, showing that electronic delocalization occurs through quantum interference between bound and ionized holong doublon pairs. © 2011 Macmillan Publishers Limited. All rights reserved.Applications of Raman scattering in quantum technologies
AIP Conference Proceedings 1267 (2010) 37-38
Coherent optical memory with GHz bandwidth
Optics InfoBase Conference Papers (2010)
Abstract:
We demonstrate the coherent storage and retrieval of sub-nanosecond low-intensity light pulses with spectral bandwidths exceeding 1 GHz in cesium vapor, using the novel, far off-resonant two-photon Raman memory protocol. © 2010 Optical Society of America.Quantum interference between photo-excited states in a solid-state mott insulator
Optics InfoBase Conference Papers (2010)
Abstract:
By exciting with sub-10-fs 1.6-μm pulses the quasi-one-dimensional Mott insulator ETF2TCNQ, we observe prompt collapse of the Mott gap modulated by 24-THz oscillations of the gap, which are assigned to quantum interference between holon-doublon excitations. © 2010 Optical Society of America.Long-distance entanglement generation in two-dimensional networks
Physical Review A - Atomic, Molecular, and Optical Physics 82:4 (2010)