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MicroPL optical setup

Professor Robert Taylor

Emeritus Professor of Condensed Matter Physics

Research theme

  • Photovoltaics and nanoscience

Sub department

  • Condensed Matter Physics

Research groups

  • Quantum Optoelectronics
Robert.Taylor@physics.ox.ac.uk
Telephone: 01865 (2)72230
Clarendon Laboratory, room 164
orcid.org/0000-0003-2578-9645
  • About
  • Teaching
  • Positions available
  • Publications

Lasing in perovskite nanocrystals

Image of transverse modes from lasing nanocrystals
Nano Research, 14, 108, 2021

Cavity-enhanced blue single-photon emission from a single InGaNGaN quantum dot

Applied Physics Letters 91:5 (2007)

Authors:

AF Jarjour, RA Taylor, RA Oliver, MJ Kappers, CJ Humphreys, A Tahraoui

Abstract:

The authors report on the generation of single photons in the blue spectral region from a single InGaNGaN quantum dot. The collection efficiency was enhanced by embedding the quantum dot layer in the middle of a low- Q microcavity. The microphotoluminescence is observed to be approximately ten times stronger than typical InGaN quantum dot emission without a cavity. The measurements were performed using nonlinear excitation spectroscopy in order to suppress the background emission from the underlying wetting layer. © 2007 American Institute of Physics.
More details from the publisher

Magneto-optical studies of single-wall carbon nanotubes

Physical Review B - Condensed Matter and Materials Physics 76:8 (2007)

Authors:

IB Mortimer, LJ Li, RA Taylor, GLJA Rikken, O Portugall, RJ Nicholas

Abstract:

We report a detailed study of the magnetophotoluminescence of single-wall carbon nanotubes at various temperatures in fields up to 58 T. We give direct experimental evidence of the diameter dependence of the Aharanov-Bohm phase-induced band gap shifts. Large increases in intensity are produced by the magnetic field at low temperatures which are also significantly chiral index [(n,m)] dependent. These increases are attributed to the magnetic field induced mixing of the wave functions of the exciton states. A study of the emission from nanotubes aligned perpendicular to the applied magnetic field shows even larger field-induced photoluminescence intensity enhancements and unexpectedly large redshifts in band gap energies, not predicted theoretically. © 2007 The American Physical Society.
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Progress in the optical studies of single InGaN/GaN quantum dots

Philosophical Magazine 87:13 (2007) 2077-2093

Authors:

AF Jarjour, RA Oliver, RA Taylor

Abstract:

The great success that GaN-based structures have enjoyed in implementing efficient optoelectronic devices has fostered a rapidly expanding interest amongst researchers aimed at understanding their underlying physics. There has been an active debate on the mechanisms that give rise to efficient luminescence in these materials. In this paper we approach these questions through optical studies of single InGaN/GaN quantum dots in the context of the available experimental and theoretical understanding of InGaN structures in general, and of three-dimensional localization in this material in particular. We will also show how it is possible to exploit the various unique properties that nitride-based materials offer, such as the strong inbuilt electric field, in a controlled manner. Such control may in the future prove essential for the implementation of single quantum dot devices in applications such as quantum information processing. We also show how nonlinear spectroscopy provides an invaluable tool in suppressing background luminescence effects inherent in this material.
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Materials challenges for devices based on single, self-assembled InGaN quantum dots

Journal of Physics: Conference Series 61:1 (2007) 889-893

Authors:

RA Oliver, AF Jarjour, A Tahraoui, MJ Kappers, RA Taylor, CJ Humphreys

Abstract:

Builiding on earlier studies of single InGaN quantum dots (QDs), we are considering their potential for use in blue- and green-emitting single photon sources. Envisaging a device based on a resonant cavity light emitting diode, we have studied the effect of growing QDs on an underlying AlN/GaN distributed Bragg reflector, and have shown that enhanced single QD emission may be obtained. Additionally, we have studied the effect of the growth and activation of a p-type cap on an underlying QD layer and have shown that the QDs survive the anneal process. © 2007 IOP Publishing Ltd.
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Photoluminescence properties of a single GaN nanorod with GaNAlGaN multilayer quantum disks

Applied Physics Letters 90:10 (2007)

Authors:

SN Yi, JH Na, KH Lee, AF Jarjour, RA Taylor, YS Park, TW Kang, S Kim, DH Ha, G Andrew, D Briggs

Abstract:

Photoluminescence (PL) properties of a single nanorod containing multiple GaN quantum disks separated by AlGaN potential barriers are investigated using micro-PL spectroscopy. Previous studies reported ensemble spectra from many nanorods. The PL spectra show different features depending on the region of the nanorod excited by the laser, including a sharp feature originating from the quantum disk region. The distinct differences between the PL from the different regions are discussed. The results imply that excitons are strongly confined in the quantum disks, and the authors suggest that small quantum disks can be regarded as quantum dots having a discrete density of states. © 2007 American Institute of Physics.
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