Mechanism of generation of the emission bands in the dynamic spectrum of the Crab pulsar

MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY 388:2 (2008) 873-883

Authors:

Houshang Ardavan, Arzhang Ardavan, John Singleton, Mario R Perez

Photoisomerization of a fullerene dimer

JOURNAL OF PHYSICAL CHEMISTRY C 112:8 (2008) 2802-2804

Authors:

Jinying Zhang, Kyriakos Porfyrakis, John JL Morton, Mark R Sambrook, Jeffrey Harmer, Li Xiao, Arzhang Ardavan, G Andrew D Briggs

Temperature-dependent photoluminescence study of ErSC2N@C80 and Er2ScN@C80 fullerenes

PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS 245:10 (2008) 1998-2001

Authors:

Archana Tiwari, Geraldine Dantelle, Kyriakos Porfyrakis, Arzhang Ardavan, G Andrew D Briggs

Configuration-selective spectroscopic studies of Er3+ centers in ErSc2N@C80 and Er2ScN@C80 fullerenes.

J Chem Phys 127:19 (2007) 194504

Authors:

Archana Tiwari, Geraldine Dantelle, Kyriakos Porfyrakis, Robert A Taylor, Andrew AR Watt, Arzhang Ardavan, G Andrew D Briggs

Abstract:

Low temperature photoluminescence (PL) and photoluminescence excitation (PLE) spectroscopy of high purity ErSc(2)N@C(80) and Er(2)ScN@C(80) fullerenes reveal at least two metastable configurations of the Er(3+) ion within the cage, consistent with previous observations from x-ray diffraction. Using PLE measurements at a number of different emission wavelengths we have characterized the ground state, (4)I(152), and the first excited state, (4)I(132), of the various Er(3+) configurations and their crystal-field splitting. We present detailed energy level diagrams for the ground and excited states of the two dominant configurations of ErSc(2)N@C(80) and Er(2)ScN@C(80).

Manipulation of quantum information in N@C60 using electron and nuclear magnetic resonance

Physica Status Solidi (B) Basic Research 244:11 (2007) 3874-3878

Authors:

A Ardavan, JJL Morton, SC Benjamin, K Porfyrakis, GAD Briggs, AM Tyryshkin, SA Lyon

Abstract:

We review recent progress towards implementing quantum information processing protocols using electron and nuclear magnetic resonance in the molecule 14N@C60. Using conventional spectrometers, we measure the errors inherent in quantum manipulations of spins. By applying composite pulses, we correct the dominant error to a high degree. Identifying a two qubit computational basis out of the electron and nuclear spin levels of 14N@C60, we implement an ultrafast phase gate on the nuclear qubit by exciting an electron spin transition. © 2007 WILEY-VCH Verlag GmbH & Co. KGaA.