Quantum spin dynamics

Abstract:

On cooling through the transition temperature Tc of a conventional superconductor, an energy gap develops as the normal-state charge carriers form Cooper pairs; these pairs form a phase-coherent condensate that exhibits the well-known signatures of superconductivity: zero resistivity and the expulsion of magnetic flux (the Meissner effect). However, in many unconventional superconductors, the formation of the energy gap is not coincident with the formation of the phase-coherent superfluid. Instead, at temperatures above the critical temperature a range of unusual properties, collectively known as 'pseudogap phenomena', are observed. Here we argue that a key pseudogap phenomenon-fluctuating superconductivity occurring substantially above the transition temperature-could be induced by the proximity of a Mott-insulating state. The Mott-insulating state in the κ-(BEDT-TTF) 2X organic molecular metals can be tuned, without doping, through superconductivity into a normal metallic state as a function of the parameter t/U, where t is the tight-binding transfer integral characterizing the metallic bandwidth and U is the on-site Coulomb repulsion. By exploiting a particularly sensitive probe of superconducting fluctuations, the vortex-Nernst effect, we find that a fluctuating regime develops as t/U decreases and the role of Coulomb correlations increases. ©2007 Nature Publishing Group.

Abstract:

We present experimental evidence for a hitherto unconfirmed type of angle-dependent magnetoresistance oscillation caused by magnetic breakdown. The effect was observed in the organic superconductor κ- (BEDT-TTF)2 Cu (NCS)2 using hydrostatic pressures of up to 9.8 kbar and magnetic fields of up to 33 T. In addition, we show that similar oscillations are revealed in ambient-pressure measurements, provided that the Shubnikov-de Haas oscillations are suppressed either by elevated temperatures or filtering of the data. These results provide a compelling validation of Pippard's semiclassical picture of magnetic breakdown. © 2007 The American Physical Society.

Abstract:

We examine environmental effects of surrounding nuclear spins on the electron spin relaxation of the N@ C60 molecule (which consists of a nitrogen atom at the center of a fullerene cage). Using dilute solutions of N@ C60 in regular and deuterated toluene, we observe and model the effect of translational diffusion of nuclear spins of the solvent molecules on the N@ C60 electron spin relaxation times. We also study spin relaxation in frozen solutions of N@ C60 in C S2, to which small quantities of a glassing agent, S2 Cl2, are added. At low temperatures, spin relaxation is caused by spectral diffusion of surrounding nuclear Cl 35,37 spins in the S2 Cl2, but, nevertheless, at 20 K, T2 as long as 0.23 ms is observed. © 2007 The American Physical Society.

Abstract:

We consider the nonspherically decaying radiation field that is generated by a polarization current with a superluminally rotating distribution pattern in vacuum, a field that decays with the distance R(P) from its source as R(P)(-1/2), instead of R(P)(-1). It is shown (i) that the nonspherical decay of this emission remains in force at all distances from its source independently of the frequency of the radiation, (ii) that the part of the source that makes the main contribution toward the value of the nonspherically decaying field has a filamentary structure whose radial and azimuthal widths become narrower (as R(P)(-2) and R(P)(-3), respectively) the farther the observer is from the source, (iii) that the loci on which the waves emanating from this filament interfere constructively delineate a radiation subbeam that is nondiffracting in the polar direction, (iv) that the cross-sectional area of each nondiffracting subbeam increases as R(P), instead of R(P)(2), so that the requirements of conservation of energy are met by the nonspherically decaying radiation automatically, and (v) that the overall radiation beam within which the field decays nonspherically consists, in general, of the incoherent superposition of such coherent nondiffracting subbeams. These findings are related to the recent construction and use of superluminal sources in the laboratory and numerical models of the emission from them. We also briefly discuss the relevance of these results to the giant pulses received from pulsars.