Andrea Cavalleri

Abstract:

A number of experiments have evidenced signatures of enhanced superconducting correlations after photoexcitation. Initially, these experiments were interpreted as resulting from quasi-static changes in the Hamiltonian parameters, for example, due to lattice deformations or melting of competing phases. Yet, several recent observations indicate that these conjectures are either incorrect or do not capture all the observed phenomena, which include reflectivity exceeding unity, large shifts of Josephson plasmon edges, and appearance of new peaks in terahertz reflectivity. These observations can be explained from the perspective of a Floquet theory involving a periodic drive of system parameters, but the origin of the underlying oscillations remains unclear. In this paper, we demonstrate that following incoherent photoexcitation, long-lived oscillations are generally expected in superconductors with low-energy Josephson plasmons, such as in cuprates or fullerene superconductor K3C60. These oscillations arise from the parametric generation of plasmon pairs due to pump-induced perturbation of the superconducting order parameter. We show that this bi-plasmon response can persist even above the transition temperature as long as strong superconducting fluctuations are present. Our analysis offers a robust framework to understand light-induced superconducting behavior, and the predicted bi-plasmon oscillations can be directly detected using available experimental techniques.

Abstract:

The interplay between charge order and superconductivity remains one of the central themes of research in quantum materials. In the case of cuprates, the coupling between striped charge fluctuations and local electromagnetic fields is especially important, as it affects transport properties, coherence, and dimensionality of superconducting correlations. Here, we study the emission of coherent terahertz radiation in single-layer cuprates of the La_2-xBa_xCuO₄ family, for which this effect is expected to be forbidden by symmetry. We find that emission vanishes for compounds in which the stripes are quasi-static but is activated when c-axis inversion symmetry is broken by incommensurate or fluctuating charge stripes, such as in La_1.905Ba_0.095CuO₄ and in La_1.845Ba_0.155CuO₄. In this case, terahertz radiation is emitted by surface Josephson plasmons, which are generally dark modes, but couple to free space electromagnetic radiation because of the stripe modulation.

Abstract:

In cuprate high-Tc superconductors, resonant excitation of certain lattice vibrations has been shown to induce transient terahertz reflectivity features suggestive of nonequilibrium superconductivity above the critical temperature Tc. A microscopic mechanism for these observations is still lacking. Here, time-resolved measurements of scattering-angle- and polarization-dependent second-harmonic generation in driven YBa2Cu3O6+x reveal a three-order-of-magnitude amplification of a 2.5-THz electronic mode, which is unique because of its symmetry, momentum, and temperature dependence. A theory for amplification of finite-momentum Josephson plasma polaritons, which are assumed to be well formed below Tc but incoherent throughout the pseudogap phase, explains all these observations. A theoretical solution for the Fresnel-Floquet reflection that starts from the coherently oscillating Josephson plasma polaritons provides a possible mechanism for the nonequilibrium superconductorlike terahertz reflectivity reported earlier. Beyond the immediate case of cuprates, this work underscores the role of nonlinear mode mixing to amplify fluctuating modes above the transition temperature in a wide range of materials.

Abstract:

An important goal of modern condensed-matter physics involves the search for states of matter with emergent properties and desirable functionalities. Although the tools for material design remain relatively limited, notable advances have been recently achieved by controlling interactions at heterointerfaces, precise alignment of low-dimensional materials and the use of extreme pressures. Here we highlight a paradigm based on controlling light–matter interactions, which provides a way to manipulate and synthesize strongly correlated quantum matter. We consider the case in which both electron–electron and electron–photon interactions are strong and give rise to a variety of phenomena. Photon-mediated superconductivity, cavity fractional quantum Hall physics and optically driven topological phenomena in low dimensions are among the frontiers discussed in this Perspective, which highlights a field that we term here ‘strongly correlated electron–photon science’.