Ian Walmsley

Abstract:

High Harmonic generation can be used as a probe of the emitting medium with attosecond and Angström resolutions. We show that polarization-resolved pump-probe spectroscopy with high harmonics improves the detection sensitivity of rotationally excited molecules.

Abstract:

The ability to store multiple optical modes in a quantum memory allows for increased efficiency of quantum communication and computation. Here we compute the multimode capacity of a variety of quantum memory protocols based on light storage in ensembles of atoms. We find that adding a controlled inhomogeneous broadening improves this capacity significantly.

Abstract:

A technique to measure the decoherence time of optical phonons in a solid is presented. Phonons are excited with a pair of time-delayed 80 fs near infrared pulses via spontaneous transient Raman scattering. The spectral fringe visibility of the resulting Raman pulse pair, as a function of time delay, is used to measure the phonon dephasing time. The method avoids the need to use either narrow band or few femtosecond pulses and is useful for low phonon excitations. The dephasing time of phonons created in bulk diamond is measured to be τ=6.8 ps (Δν=1.56 cm-1). ©2008 The American Physical Society.