Oxford Centre for High Energy Density Science (OxCHEDS)

Abstract:

The recovery of metastable structures formed at high pressure has been a long-standing goal in the field of condensed matter physics. While laser-driven compression has been used as a method to generate novel structures at high pressure, to date no high-pressure phases have been quenched to ambient conditions. Here we demonstrate, using in situ x-ray diffraction and recovery methods, the successful quench of a high-pressure phase which was formed under laser-driven shock compression. We show that tailoring the pressure release path from a shock-compressed state to eliminate sample spall, and therefore excess heating, increases the recovery yield of the high-pressure ω phase of zirconium from 0% to 48%. Our results have important implications for the quenchability of novel phases of matter demonstrated to occur at extreme pressures using nanosecond laser-driven compression.

Abstract:

Hydrodynamic optical-field-ionised (HOFI) plasma channels promise a route towards high repetition-rate, metre-scale stages for future laser plasma accelerators. These channels are formed by hydrodynamic expansion of a plasma column produced by optical field ionisation at the focus of a laser, typically from an axicon lens. Since the laser pulses used to generate the initial plasma column are of sub-picosecond duration, chromatic effects in the axicon lens could be important. In this paper we assess these effects using a numerical propagation code. The code is validated using analytical formulae and experimental data. For the parameter range investigated, dispersive effects are found to be of minor importance, reducing the peak on-axis intensity in the focal region by approximately 10%.