Quantum interference between charge excitation paths in a solid-state Mott insulator

Nature Physics 7:2 (2011) 114-118

Authors:

S Wall, D Brida, SR Clark, HP Ehrke, D Jaksch, A Ardavan, S Bonora, H Uemura, Y Takahashi, T Hasegawa, H Okamoto, G Cerullo, A Cavalleri

Abstract:

Competition between electron localization and delocalization in Mott insulators underpins the physics of strongly correlated electron systems. Photoexcitation, which redistributes charge, can control this many-body process on the ultrafast 1,2 timescale. So far, time-resolved studies have been carried out in solids in which other degrees of freedom, such as lattice, spin or orbital excitations 3-5 , dominate. However, the underlying quantum dynamics of bareg electronic excitations has remained out of reach. Quantum many-body dynamics are observed only in the controlled environment of optical lattices 6,7 where the dynamics are slower and lattice excitations are absent. By using nearly single-cycle near-infrared pulses, we have measured coherent electronic excitations in the organic salt ET-F 2 TCNQ, a prototypical one-dimensional Mott insulator. After photoexcitation, a new resonance appears, which oscillates at 25THz. Time-dependent simulations of the Mottg Hubbard Hamiltonian reproduce the oscillations, showing that electronic delocalization occurs through quantum interference between bound and ionized holong doublon pairs. © 2011 Macmillan Publishers Limited. All rights reserved.

Applications of Raman scattering in quantum technologies

AIP Conference Proceedings 1267 (2010) 37-38

Authors:

KF Reim, P Bustard, KC Lee, J Nunn, VO Lorenz, BJ Sussman, NK Langford, D Jaksch, IA Walmsley

Coherent optical memory with GHz bandwidth

Optics InfoBase Conference Papers (2010)

Authors:

KF Reim, J Nunn, VO Lorenz, BJ Sussman, KC Lee, NK Langford, D Jaksch, IA Walmsley

Abstract:

We demonstrate the coherent storage and retrieval of sub-nanosecond low-intensity light pulses with spectral bandwidths exceeding 1 GHz in cesium vapor, using the novel, far off-resonant two-photon Raman memory protocol. © 2010 Optical Society of America.

Quantum interference between photo-excited states in a solid-state mott insulator

Optics InfoBase Conference Papers (2010)

Authors:

S Wall, D Brida, SR Clark, HP Ehrke, D Jaksch, A Ardavan, S Bonora, H Uemura, Y Takahashi, T Hasegawa, H Okamoto, G Cerullo, A Cavalleri

Abstract:

By exciting with sub-10-fs 1.6-μm pulses the quasi-one-dimensional Mott insulator ETF2TCNQ, we observe prompt collapse of the Mott gap modulated by 24-THz oscillations of the gap, which are assigned to quantum interference between holon-doublon excitations. © 2010 Optical Society of America.

Long-distance entanglement generation in two-dimensional networks

Physical Review A - Atomic, Molecular, and Optical Physics 82:4 (2010)

Authors:

S Broadfoot, U Dorner, D Jaksch

Abstract:

We consider two-dimensional networks composed of nodes initially linked by two-qubit mixed states. In these networks we develop a global error correction scheme that can generate distance-independent entanglement from arbitrary network geometries using rank-2 states. By using this method and combining it with the concept of percolation, we also show that the generation of long-distance entanglement is possible with rank-3 states. Entanglement percolation and global error correction have different advantages depending on the given situation. To reveal the trade-off between them we consider their application to networks containing pure states. In doing so we find a range of pure-state schemes, each of which has applications in particular circumstances: For instance, we can identify a protocol for creating perfect entanglement between two distant nodes. However, this protocol cannot generate a singlet between any two nodes. In contrast, we can also construct schemes for creating entanglement between any nodes, but the corresponding entanglement fidelity is lower. © 2010 The American Physical Society.