Switching of ferrotoroidal domains via an intermediate mixed state in the multiferroic Y-type hexaferrite Ba0.5Sr1.5Mg2Fe12O22
Abstract:
We report a detailed study of the magnetic field switching of ferrotoroidal/multiferroic domains in the Y-type hexaferrite compound Ba0.5Sr1.5Mg2Fe12O22. By combining data from superconducting quantum interference device (SQUID) magnetometry, magnetocurrent measurements, and resonant x-ray scattering experiments, we arrive at a complete description of the deterministic switching, which involves the formation of a temperaturedependent mixed state in low magnetic fields. This mechanism is likely to be shared by other members of the hexaferrite family, and presents a challenge for the development of high-speed read-write memory devices based on these materials.
Characterizing the diffuse continuum excitations in the classical spin liquid h-YMnO3
Spin dynamics and possible topological magnons in the nonstoichiometric pyrochlore iridate Tb2Ir2O7 studied by RIXS
Strain-induced antiferromagnetic domain switching via the spin Jahn-Teller effect
A multimodal approach reveals the symmetry-breaking pathway to the broken helix in EuIn2As2
Abstract:
Understanding and manipulating emergent phases, which are themes at the forefront of quantum-materials research, rely on identifying their underlying symmetries. This general principle has been particularly prominent in materials with coupled electronic and magnetic degrees of freedom, in which magnetic order influences the electronic band structure and can lead to exotic topological effects. However, identifying symmetry of a magnetically ordered phase can pose a challenge, particularly in the presence of small domains. Here we introduce a multimodal approach for determining magnetic structures, which combines symmetry-sensitive optical probes, scattering, and group-theoretical analysis. We apply it to EuIn2As2, a material that has received attention as a candidate axion insulator. While first-principles calculations predict this state on the assumption of a simple collinear antiferromagnetic structure, subsequent neutron-scattering measurements reveal a much more intricate magnetic ground state characterized by two coexisting magnetic wave vectors reached by successive thermal phase transitions. The proposed high- and low-temperature phases are a spin helix and a state with interpenetrating helical and Néel antiferromagnetic order termed a “broken helix,” respectively. Employing a multimodal approach, we identify the magnetic structure associated with these two phases of EuIn2As2. We find that the higher-temperature phase is characterized by a variation of the magnetic moment amplitude from layer to layer, with the moment vanishing entirely in every third Eu layer. The lower-temperature structure is similar to the broken helix, with one important difference: Because of local strain, the relative orientation of the magnetic structure and the lattice is not fixed. Consequently, the symmetry required to protect the axion phase is not generically protected in EuIn2As2, but we show that it can be restored if the magnetic structure is tuned with uniaxial strain. Finally, we present a spin Hamiltonian that identifies the spin interactions that account for the complex magnetic order in EuIn2As2. Our work highlights the importance of a multimodal approach in determining the symmetry of complex order parameters.