Thin film quantum materials

Abstract:

Abstract:

Breaking time-reversal symmetry through magnetic doping of topological insulators has been identified as a key strategy for unlocking exotic physical states. Here, we report the growth of Bi2Te3 thin films doped with the highest magnetic moment element Ho. Diffraction studies demonstrate high quality films for up to 21% Ho incorporation. Superconducting quantum interference device magnetometry reveals paramagnetism down to 2 K with an effective magnetic moment of ∼5 μB/Ho. Angle-resolved photoemission spectroscopy shows that the topological surface state remains intact with Ho doping, consistent with the material's paramagnetic state. The large saturation moment achieved makes these films useful for incorporation into heterostructures, whereby magnetic order can be introduced via interfacial coupling.

Abstract:

By coupling magnetic elements to metamaterials, hybrid metamolecules can be created with useful properties such as photon-magnon mode mixing. Here, we present results for a split-ring resonator (SRR) placed in close proximity to a thin crystalline film of magnetically hard FeCo. Eddy-current shielding is suppressed by patterning the FeCo into 100-μm disks. At the ferromagnetic resonance (FMR) condition of FeCo, photon-magnon coupling strengths of 5% are observed. Altogether, three distinct features are presented and discussed: (i) remanent magnets allow FMR to be performed in a near-zero field, partially eliminating the need for applied fields; (ii) the anisotropic FMR permits angular control over hybrid SRR and FMR resonances; and (iii) the in-plane and out-of-plane magnetization of FeCo opens the door to “magnetically configurable metamaterials” in real time. Finally, a special study is presented of how best to excite the numerous transverse magnetic and electric modes of the SRR by using near-field excitation from a coplanar waveguide.