Prof Peter Norreys FInstP;

Abstract:

Bright harmonic radiation from relativistically oscillating laser plasmas offers a direct route for generating extreme electromagnetic fields. Theory predicts that under optimized conditions, the plasma medium can support strong spatiotemporal compression of laser energy in a coherent harmonic focus (CHF), delivering intensity boosts many orders of magnitude greater than the incident driving laser pulse^1,2,3,4. Although diffraction-limited performance⁵ (spatial compression) and attosecond phase locking^6,7,8 (temporal compression) have been demonstrated experimentally, efficient coupling of relativistically intense laser pulse energy into the emitted harmonic cone has not been realized so far. Here we demonstrate that this highly nonlinear interaction can be tailored to deliver the maximum conversion efficiencies predicted from simulations. By fine-tuning the temporal profile of the driving laser on sub-picosecond (<10⁻¹² s) timescales, energies >9 mJ between the 12th and 47th harmonics are observed. These results are in agreement with the theoretically expected efficiency dependence on harmonic order, verifying that optimal conditions have been achieved in the generation process. This is the important final element required to achieve the expected intensity boosts from a CHF in experiments. Although obtaining spatiotemporal compression and optimal efficiency simultaneously remains challenging, the path to realizing extreme optical field strengths approaching the critical field of quantum electrodynamics (the Schwinger limit at >10¹⁶ V cm⁻¹ or >10²⁹ W cm⁻²) is now open, permitting all-optical studies of the quantum vacuum and new frontiers for intense attosecond science.

Abstract:

We introduce a Bayesian framework for measuring spatio-temporal couplings (STCs) in ultra-intense lasers that reconceptualizes what constitutes a ’single-shot’ measurement. Moving beyond traditional distinctions between single- and multi-shot devices, our approach provides rigorous criteria for determining when measurements can truly resolve individual laser shots rather than statistical averages. By contextualizing single measurements, this framework shows that single-shot capability is not an intrinsic device property but emerges from the relationship between measurement precision and predictability. Implementing this approach with a new measurement device at the ATLAS-3000 petawatt laser, we provide the first quantitative uncertainty bounds on pulse front tilt and curvature. Notably, we observe that our Bayesian method reduces uncertainty by up to 60% compared to traditional approaches. Through this analysis, we reveal how the interplay between measurement precision and intrinsic system variability defines achievable resolution—insights that have direct implications for applications where precise control of laser-matter interaction is critical.

Abstract:

The control of light’s various degrees of freedom underpins modern physics and technology, from quantum optics to telecommunications. Ultraintense lasers represent the pinnacle of this control, concentrating light to extreme intensities at which electrons oscillate at relativistic velocities within a single optical cycle. These extraordinary conditions offer unique opportunities to probe the fundamental aspects of light–matter interactions and develop transformative applications. However, the precise characterization of intense, ultrashort lasers has lagged behind our ability to generate them, creating a bottleneck in advancing laser science and its applications. Here we present the first single-shot vector field measurement technique for intense, ultrashort laser pulses that provides an unprecedented insight into their complete spatiotemporal and polarization structure, including quantified uncertainties. Our method efficiently encodes the full vector field onto a two-dimensional detector by leveraging the inherent properties of these laser pulses, allowing for real-time characterization. We demonstrate its capabilities on systems ranging from high-repetition-rate oscillators to petawatt-class lasers, revealing subtle spatiotemporal couplings and polarization effects. This advancement bridges the gap between theory and experiment in laser physics, providing crucial data for simulations and accelerating the development of novel applications in high-field physics, laser–matter interactions, future energy solutions and beyond.

Abstract:

The global commissioning of multi-Petawatt laser systems provides unprecedented access to ultra-high electromagnetic fields for probing the quantum vacuum. However, current analytical models are limited, necessitating large-scale simulations for experimental validation. Here, we present real-time three-dimensional simulations of two quantum vacuum effects, using a semi-classical numerical solver based on the Heisenberg-Euler Lagrangian. The simulation model is benchmarked against vacuum birefringence analytical results with a counter-propagating setup. Simulations results of both plane-wave and Gaussian pulses are consistent with theoretical predictions. The solver is then applied to four-wave mixing using three Gaussian pulses with real-time information on the harmonic evolution. We provide quantitative explanations for the astigmatism in the output and produce precise estimates of the interaction time and size. Results are compared with the plane-wave model and previous numerical results. This solver paves the way for in-depth investigations of a broad spectrum of quantum vacuum effects in any arbitrary laser setup.