Electronic structures and photoemission spectroscopy

Abstract:

Band renormalizations comprise crucial insights for understanding the intricate roles of electron-boson coupling and electron correlation in emergent phenomena such as superconductivity. In this Letter, by combining high-resolution angle-resolved photoemission spectroscopy and theoretical calculations, we systematically investigate the electronic structure of the trilayer nickelate superconductor La_{4}Ni_{3}O_{10} at ambient pressure. We reveal a dichotomy in the electronic band renormalizations of La_{4}Ni_{3}O_{10} in comparison to cuprate superconductors. At a high energy scale of hundreds of meV, its band structure is strongly renormalized by an electron correlation effect enhanced by Hund's coupling. The resultant waterfall-like dispersions resemble the high-energy kinks in cuprate superconductors. However, at low-energy scales of tens of meV, the dispersive bands are nearly featureless and devoid of any resolvable electron-boson interactions, in drastic contrast to the low-energy kinks observed in cuprates and other correlated 3d transition-metal compounds. The dichotomic band renormalizations highlight the disparity between nickelate and cuprate superconductors and emphasize the importance of strong electron correlation in the superconductivity of Ruddlesden-Popper phase nickelates.

Abstract:

The recently discovered heavy-fermion superconductor, UTe2, is an excellent candidate for spin-triplet superconductors in which electrons form spin-triplet Cooper pairs with spin S = 1 and odd parity. Unconventional superconductivity often hosts unconventional vortices. Yet, the vortex core and lattice in UTe2 have not been directly visualized and characterized. Here, by using ultralow-temperature scanning tunnelling microscopy and spectroscopy, we study the superconducting vortices on the (0−11) surface termination of UTe2 with an out-of-plane external magnetic field. At the centre of the vortex core, we observe a robust zero-energy vortex-core state that exhibits a cigar-shaped spatial distribution and extends to ∼30 nm along the [100] direction (crystallographic a-axis) of UTe2. Along the direction perpendicular to [100], the superconducting gap is deeper and the coherence peak on one side of the vortex core is stronger than on the opposite side, and they are even enhanced in comparison with those under zero field. Due to the anisotropy of magnetic susceptibility in UTe2, the asymmetric dI/dV spectra on the two sides of the vortex core result from the interplay between the magnetization-induced bound current and supercurrent around the vortex core. Our work reveals the important role of magnetization in the vortex behaviours of UTe2 and provides essential microscopic information for understanding its superconducting properties in a magnetic field.

Abstract:

PrAlSi, a non‐centrosymmetric ferromagnetic Weyl semimetal candidate with a Curie temperature of 17.8K, offers a unique platform for exploring the interplay of symmetry breaking and topological electronic structures. Up to now, the Weyl fermion distribution as well as their evolution across the ferromagnetic to paramagnetic phase transition in PrAlSi has not been explored. Here, the presence of Weyl fermions is uncovered in PrAlSi and demonstrates that they can be manipulated through the magnetic phase transition. The ab‐initio calculations indicate a shift in the momentum and energy positions of Weyl fermions, alongside an increase in Weyl point numbers due to band splitting. The predicted band splitting and shifting of Weyl fermions are corroborated by the angle‐resolved photoemission spectroscopy experiments. Such manipulation of Weyl fermions leads to the appearance of a net chirality charge and a significant modulation in optical conductivity, as proposed by the calculations. The research presents a novel method for adjusting the properties of Weyl semimetals by controlling Weyl fermions through magnetic phase transitions, positioning PrAlSi as a model system.

Abstract:

Correlated kagome materials exhibit a compelling interplay between lattice geometry, electron correlation, and topology. In particular, the flat bands near the Fermi level provide a fertile playground for novel many-body states. Here we investigate the electronic structure of CsCr3Sb5 using high-resolution angle-resolved photoemission spectroscopy and ab-initio calculations. Our results suggest that Cr 3d electrons are intrinsically incoherent, showing strong electron correlation amplified by Hund’s coupling. Notably, we identify incipient flat bands close to the Fermi level, which are expected to significantly influence the electronic properties of the system. Across the density-wave-like transition at 55 K, we observe a drastic enhancement of the electron scattering rate, which aligns with the semiconducting-like property at high temperatures. These findings establish CsCr3Sb5 as a strongly correlated Hund’s metal with incipient flat bands near the Fermi level, which provides an electronic basis for understanding its novel properties compared to the weakly correlated AV3Sb5.