Muons and magnets

Abstract:

Chiral magnets are promising materials for the realisation of high-density and low-power spintronic memory devices. For these future applications, a key requirement is the synthesis of appropriate materials in the form of thin films ordering well above room temperature. Driven by the Dzyaloshinskii-Moriya interaction, the cubic compound FeGe exhibits helimagnetism with a relatively high transition temperature of 278K in bulk crystals. We demonstrate that this temperature can be enhanced significantly in thin films. Using x-ray spectroscopic and ferromagnetic resonance techniques, we provide unambiguous experimental evidence for long-wavelength helimagnetic order at room temperature and magnetic properties similar to the bulk material. We obtain αintr = 0:0036 ± 0:0003 at 310K for the intrinsic damping parameter. We probe the dynamics of the system by means of muon-spin rotation, indicating that the ground state is reached via a freezing out of slow dynamics. Our work paves the way towards the fabrication of thin films of chiral magnets that host certain spin whirls, so-called skyrmions, at room temperature and potentially offer integrability into modern electronics.

Abstract:

We demonstrate that quantum-critical spin dynamics can be probed in high magnetic fields using muon-spin relaxation (μ+SR). Our model system is the strong-leg spin ladder bis(2,3-dimethylpyridinium) tetrabromocuprate (DIMPY). In the gapless Tomonaga-Luttinger liquid phase we observe finite-temperature scaling of the μ+SR 1/T1 relaxation rate which allows us to determine the Luttinger parameter K. We discuss the benefits and limitations of local probes compared with inelastic neutron scattering.