Resonance-Amplified Terahertz Near-Field Spectroscopy of a Single Nanowire.

Nano letters 24:49 (2024) 15716-15723

Authors:

Sarah Norman, Greg Chu, Kun Peng, James Seddon, Lucy L Hale, Hark Hoe Tan, Chennupati Jagadish, Ralf Mouthaan, Jack Alexander-Webber, Hannah J Joyce, Michael B Johnston, Oleg Mitrofanov, Thomas Siday

Abstract:

Nanoscale material systems are central to next-generation optoelectronic and quantum technologies, yet their development remains hindered by limited characterization tools, particularly at terahertz (THz) frequencies. Far-field THz spectroscopy techniques lack the sensitivity for investigating individual nanoscale systems, whereas in near-field THz nanoscopy, surface states, disorder, and sample-tip interactions often mask the response of the entire nanoscale system. Here, we present a THz resonance-amplified near-field spectroscopy technique that can detect subtle conductivity changes in isolated nanoscale systems─such as a single InAs nanowire─under ultrafast photoexcitation. By exploiting the spatial localization and resonant field enhancement in the gap of a bowtie antenna, our approach enables precise measurements of the nanostructures through shifts in the antenna resonant frequency, offering a direct means of extracting the system response, and unlocking investigations of ultrafast charge-carrier dynamics in isolated nanoscale and microscale systems.

A thorough experimental assessment of THz-TDS plasma diagnostic techniques for nuclear fusion applications.

The Review of scientific instruments 95:10 (2024) 103519

Authors:

G Galatola Teka, K Peng, M Alonzo, F Bombarda, CL Koch-Dandolo, L Senni, A Taschin, M Zerbini

Abstract:

In this paper, the study of a plasma diagnostic system based on the THz time domain spectroscopy technique is presented. Such a system could potentially probe a large part of the electromagnetic spectrum currently covered by several other diagnostics in a single measurement. This feature, keeping in mind the basic requirements for plasma diagnostics in nuclear fusion experiments, such as robustness and hard environment applicability, as well as durability and low maintenance, makes the diagnostic of great interest. A conceptual design of the THz-TDS diagnostic has been developed, starting from the well-established classical microwave and far infrared plasma diagnostics landscape. The physical constraints and required instrumental characteristics have been studied and are described in detail here, together with the solutions available for each type of plasma measurement. Specific experimental laboratory tests of the different experimental configurations have been carried out, evaluating the capacity and potential of the novel diagnostic, together with the instrumental constraint, within the diagnostic parameter space.

Alumina nanoparticles enable optimal spray-coated perovskite thin film growth on self-assembled monolayers for efficient and reproducible photovoltaics

Journal of Materials Chemistry C Royal Society of Chemistry (RSC) 12:34 (2024) 13332-13342

Authors:

Elena J Cassella, Robert DJ Oliver, Timothy Thornber, Sophie Tucker, Rehmat Goodwin, David G Lidzey, Alexandra J Ramadan

Roadmap on established and emerging photovoltaics for sustainable energy conversion

Journal of Physics Energy IOP Publishing (2024)

Authors:

James C Blakesley, Ruy Sebastian Bonilla, Marina Freitag, Alex Ganose, Nicola Gasparini, Pascal Kaienburg, George Koutsourakis, Jonathan D Major, Jenny Nelson, Nakita K Noel, Bart Roose, Jae Sung Yun, Simon Aliwell, Pietro Altermatt, Tayebeh Ameri, Virgil Andrei, Ardalan Armin, Diego Bagnis, Jenny Baker, Hamish Beath, Mathieu Bellanger, Philippe Berrouard, Jochen Blumberger, Stuart Boden, Hugo Bronstein, Matthew J Carnie, Chris Case, Fernando A Castro, Yi-Ming Chang, Elmer Chao, Tracey M Clarke, Graeme Cooke, Pablo Docampo, Ken Durose, James Durrant, Marina Filip, Richard H Friend, Jarvist M Frost, Elizabeth Gibson, Alexander J Gillett, Pooja Goddard, Severin Habisreutinger, Martin Heeney, Arthur D Hendsbee, Louise Caroline Hirst, Saiful Islam, Imalka Jayawardena, Michael Johnston, Matthias Kauer, Jeff Kettle

Abstract:

<jats:title>Abstract</jats:title> <jats:p>Photovoltaics (PVs) are a critical technology for curbing growing levels of anthropogenic greenhouse gas emissions, and meeting increases in future demand for low-carbon electricity. In order to fulfil ambitions for net-zero carbon dioxide equivalent (CO<jats:sub>2</jats:sub>eq) emissions worldwide, the global cumulative capacity of solar PVs must increase by an order of magnitude from 0.9 TW<jats:sub>p</jats:sub> in 2021 to 8.5 TW<jats:sub>p</jats:sub> by 2050 according to the International Renewable Energy Agency, which is considered to be a highly conservative estimate. In 2020, the Henry Royce Institute brought together the UK PV community to discuss the critical technological and infrastructure challenges that need to be overcome to address the vast challenges in accelerating PV deployment. Herein, we examine the key developments in the global community, especially the progress made in the field since this earlier roadmap, bringing together experts primarily from the UK across the breadth of the photovoltaics community. The focus is both on the challenges in improving the efficiency, stability and levelized cost of electricity of current technologies for utility-scale PVs, as well as the fundamental questions in novel technologies that can have a significant impact on emerging markets, such as indoor PVs, space PVs, and agrivoltaics. We discuss challenges in advanced metrology and computational tools, as well as the growing synergies between PVs and solar fuels, and offer a perspective on the environmental sustainability of the PV industry. Through this roadmap, we emphasize promising pathways forward in both the short- and long-term, and for communities working on technologies across a range of maturity levels to learn from each other.</jats:p>

The Role of Chemical Composition in Determining the Charge‐Carrier Dynamics in (AgI)x(BiI3)y Rudorffites

Advanced Functional Materials Wiley 34:32 (2024)

Authors:

Snigdha Lal, Marcello Righetto, Benjamin WJ Putland, Harry C Sansom, Silvia G Motti, Heon Jin, Michael B Johnston, Henry J Snaith, Laura M Herz