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A VUV sub-micron hotspot for photoemission spectroscopy

Vacuum ultraviolet (VUV) lasers have exhibited great potential as the light source for various spectroscopies, which, if they can be focused into a smaller beam spot, will not only allow investigation of mesoscopic materials but also find applications in manufacture of nano-objects with excellent precision. Towards this goal, scientists in China invented a 177 nm VUV laser system that can achieve a record-small (<1 μm) focal spot at a long focal length (~45 mm). This system can be re-equipped for usage in low-cost ARPES and might benefit quantum materials, condensed matter physics and nanophotonics.

Prof Yulin Chen

Professor of Physics

Research theme

  • Quantum materials

Sub department

  • Condensed Matter Physics

Research groups

  • Electronic structures and photoemission spectroscopy
yulin.chen@physics.ox.ac.uk
Clarendon Laboratory, room RM263, Mullard Bldg.
Recent publications
  • About
  • Publications

Distinct superconducting states in the pressure-induced metallic structures of topological heterostructure BiTe

Materials Today Physics Elsevier 42 (2024) 101377

Authors:

Shihao Zhu, Bangshuai Zhu, Cuiying Pei, Qi Wang, Jing Chen, Qinghua Zhang, Tianping Ying, Lin Gu, Yi Zhao, Changhua Li, Weizheng Cao, Mingxin Zhang, Lili Zhang, Jian Sun, Yulin Chen, Juefei Wu, Yanpeng Qi
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Distinct superconducting states in the pressure-induced metallic structures of topological heterostructure BiTe

Materials Today Physics Elsevier 42 (2024) 101377

Abstract:

The (Bi2)m(Bi2Te3)n homologous series possess natural multilayer heterostructure with intriguing physical properties at ambient pressure. Herein, we report the pressure-dependent evolution of the structure and electrical transport of the dual topological insulator BiTe, a member of the (Bi2)m(Bi2Te3)n series. With applied pressure, BiTe exhibits several different crystal structures and distinct superconducting states, which is remarkably similar to other members of the (Bi2)m(Bi2Te3)n series. Our results provide a systematic phase diagram for the pressure-induced superconductivity in BiTe, contributing to the highly interesting physics in this (Bi2)m(Bi2Te3)n series.

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Controlling charge density order in 2⁢𝐻−TaSe2 using a van Hove singularity

Physical Review Research American Physical Society 6 (2024) 013088

Authors:

Luckin, Dharmalingam Prabhakaran, Yulin Chen

Abstract:

We report on the interplay between a van Hove singularity and a charge density wave state in 2⁢𝐻−TaSe2. We use angle-resolved photoemission spectroscopy to investigate changes in the Fermi surface of this material under surface doping with potassium. At high doping, we observe modifications which imply the disappearance of the (3×3) charge density wave and formation of a different correlated state. Using a tight-binding-based approach as well as an effective model, we explain our observations as a consequence of coupling between the single-particle Lifshitz transition during which the Fermi level passes a van Hove singularity and the charge density order. In this scenario, the high electronic density of states associated with the van Hove singularity induces a change in the periodicity of the charge density wave from the known (3×3) to a new (2×2) superlattice.
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ARPES investigation of the electronic structure and its evolution in magnetic topological insulator MnBi2+2nTe4+3n family

Nature Physics Springer Nature 20:4 (2024) 571-578

Authors:

Dingsong Wu, Jiangang Yang, Jieyi Liu, Houke Chen, Yiheng Yang, Cheng Peng, Yulin Chen, Junjie Jia

Abstract:

The origin of high-temperature superconductivity in iron-based superconductors is still not understood; determination of the pairing symmetry is essential for understanding the superconductivity mechanism. In the iron-based superconductors that have hole pockets around the Brillouin zone centre and electron pockets around the zone corners, the pairing symmetry is generally considered to be s±, which indicates a sign change in the superconducting gap between the hole and electron pockets. For the iron-based superconductors with only hole pockets, however, a couple of pairing scenarios have been proposed, but the exact symmetry is still controversial. Here we determine that the pairing symmetry in KFe2As2—which is a prototypical iron-based superconductor with hole pockets both around the zone centre and around the zone corners—is also of the s± type. Our laser-based angle-resolved photoemission measurements have determined the superconducting gap distribution and identified the locations of the gap nodes on all the Fermi surfaces around the zone centres and the zone corners. These results unify the pairing symmetry in hole-doped iron-based superconductors and point to spin fluctuation as the pairing glue in generating superconductivity.
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Nodal s± pairing symmetry in an iron-based superconductor with only hole pockets

Nature Physics Springer Nature 20:4 (2024) 571-578

Authors:

Dingsong Wu, Junjie Jia, Jiangang Yang, Wenshan Hong, Yingjie Shu, Taimin Miao, Hongtao Yan, Hongtao Rong, Ping Ai, Xing Zhang, Chaohui Yin, Jieyi Liu, Houke Chen, Yiheng Yang, Cheng Peng, Chenlong Li, Shenjin Zhang, Fengfeng Zhang, Feng Yang, Zhimin Wang, Nan Zong, Lijuan Liu, Rukang Li, Xiaoyang Wang, Qinjun Peng, Hanqing Mao, Guodong Liu, Shiliang Li, Yulin Chen, Huiqian Luo, Xianxin Wu, Zuyan Xu, Lin Zhao, Xj Zhou

Abstract:

The origin of high-temperature superconductivity in iron-based superconductors is still not understood; determination of the pairing symmetry is essential for understanding the superconductivity mechanism. In the iron-based superconductors that have hole pockets around the Brillouin zone centre and electron pockets around the zone corners, the pairing symmetry is generally considered to be s±, which indicates a sign change in the superconducting gap between the hole and electron pockets. For the iron-based superconductors with only hole pockets, however, a couple of pairing scenarios have been proposed, but the exact symmetry is still controversial. Here we determine that the pairing symmetry in KFe2As2—which is a prototypical iron-based superconductor with hole pockets both around the zone centre and around the zone corners—is also of the s± type. Our laser-based angle-resolved photoemission measurements have determined the superconducting gap distribution and identified the locations of the gap nodes on all the Fermi surfaces around the zone centres and the zone corners. These results unify the pairing symmetry in hole-doped iron-based superconductors and point to spin fluctuation as the pairing glue in generating superconductivity.
More details from the publisher
Details from ORA
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