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A VUV sub-micron hotspot for photoemission spectroscopy

Vacuum ultraviolet (VUV) lasers have exhibited great potential as the light source for various spectroscopies, which, if they can be focused into a smaller beam spot, will not only allow investigation of mesoscopic materials but also find applications in manufacture of nano-objects with excellent precision. Towards this goal, scientists in China invented a 177 nm VUV laser system that can achieve a record-small (<1 μm) focal spot at a long focal length (~45 mm). This system can be re-equipped for usage in low-cost ARPES and might benefit quantum materials, condensed matter physics and nanophotonics.

Prof Yulin Chen

Professor of Physics

Research theme

  • Quantum materials

Sub department

  • Condensed Matter Physics

Research groups

  • Electronic structures and photoemission spectroscopy
yulin.chen@physics.ox.ac.uk
Clarendon Laboratory, room RM263, Mullard Bldg.
Recent publications
  • About
  • Publications

Spectroscopic evidence of symmetry breaking in the superconducting vortices of UTe 2

National Science Review Oxford University Press 12:8 (2025) nwaf267

Authors:

Zhongzheng Yang, Fanbang Zheng, Dingsong Wu, Bin-Bin Zhang, Ning Li, Wenhui Li, Chaofan Zhang, Guang-Ming Zhang, Xi Chen, Yulin Chen, Shichao Yan

Abstract:

The recently discovered heavy-fermion superconductor, UTe2, is an excellent candidate for spin-triplet superconductors in which electrons form spin-triplet Cooper pairs with spin S = 1 and odd parity. Unconventional superconductivity often hosts unconventional vortices. Yet, the vortex core and lattice in UTe2 have not been directly visualized and characterized. Here, by using ultralow-temperature scanning tunnelling microscopy and spectroscopy, we study the superconducting vortices on the (0−11) surface termination of UTe2 with an out-of-plane external magnetic field. At the centre of the vortex core, we observe a robust zero-energy vortex-core state that exhibits a cigar-shaped spatial distribution and extends to ∼30 nm along the [100] direction (crystallographic a-axis) of UTe2. Along the direction perpendicular to [100], the superconducting gap is deeper and the coherence peak on one side of the vortex core is stronger than on the opposite side, and they are even enhanced in comparison with those under zero field. Due to the anisotropy of magnetic susceptibility in UTe2, the asymmetric dI/dV spectra on the two sides of the vortex core result from the interplay between the magnetization-induced bound current and supercurrent around the vortex core. Our work reveals the important role of magnetization in the vortex behaviours of UTe2 and provides essential microscopic information for understanding its superconducting properties in a magnetic field.
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Proximity‐Induced Superconducting Diode Effect in Antiferromagnetic Mott Insulator α‐RuCl 3

Advanced Functional Materials Wiley (2025)

Authors:

Jiadian He, Yifan Ding, Xiaohui Zeng, Yiwen Zhang, Yanjiang Wang, Peng Dong, Yueshen Wu, Kecheng Cao, Kejing Ran, Xiang Zhou, Jinghui Wang, Yulin Chen, Kenji Watanabe, Takashi Taniguchi, Shun‐Li Yu, Jian‐Xin Li, Jinsheng Wen, Jun Li
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Weyl Fermion Manipulation Through Magnetic Transitions in the Ferromagnetic Non‐Centrosymmetric Weyl Semimetal PrAlSi

Advanced Electronic Materials Wiley (2025) 2500044

Authors:

Kaipu Wang, Wujun Shi, Weizheng Cao, Xiaotian Yang, Zhengyang Lv, Cheng Peng, Cheng Chen, Defa Liu, Haifeng Yang, Lexian Yang, Meng Lyu, Peijie Sun, Enke Liu, Mao Ye, Yulin Chen, Yan Sun, Yanpeng Qi, Zhongkai Liu

Abstract:

PrAlSi, a non‐centrosymmetric ferromagnetic Weyl semimetal candidate with a Curie temperature of 17.8K, offers a unique platform for exploring the interplay of symmetry breaking and topological electronic structures. Up to now, the Weyl fermion distribution as well as their evolution across the ferromagnetic to paramagnetic phase transition in PrAlSi has not been explored. Here, the presence of Weyl fermions is uncovered in PrAlSi and demonstrates that they can be manipulated through the magnetic phase transition. The ab‐initio calculations indicate a shift in the momentum and energy positions of Weyl fermions, alongside an increase in Weyl point numbers due to band splitting. The predicted band splitting and shifting of Weyl fermions are corroborated by the angle‐resolved photoemission spectroscopy experiments. Such manipulation of Weyl fermions leads to the appearance of a net chirality charge and a significant modulation in optical conductivity, as proposed by the calculations. The research presents a novel method for adjusting the properties of Weyl semimetals by controlling Weyl fermions through magnetic phase transitions, positioning PrAlSi as a model system.
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Electron correlation and incipient flat bands in the Kagome superconductor CsCr 3 Sb 5

Nature Communications Nature Research 16:1 (2025) 3229

Authors:

Yidian Li, Yi Liu, Xian Du, Siqi Wu, Wenxuan Zhao, Kaiyi Zhai, Yinqi Hu, Senyao Zhang, Houke Chen, Jieyi Liu, Yiheng Yang, Cheng Peng, Makoto Hashimoto, Donghui Lu, Zhongkai Liu, Yilin Wang, Yulin Chen, Guanghan Cao, Lexian Yang

Abstract:

Correlated kagome materials exhibit a compelling interplay between lattice geometry, electron correlation, and topology. In particular, the flat bands near the Fermi level provide a fertile playground for novel many-body states. Here we investigate the electronic structure of CsCr3Sb5 using high-resolution angle-resolved photoemission spectroscopy and ab-initio calculations. Our results suggest that Cr 3d electrons are intrinsically incoherent, showing strong electron correlation amplified by Hund’s coupling. Notably, we identify incipient flat bands close to the Fermi level, which are expected to significantly influence the electronic properties of the system. Across the density-wave-like transition at 55 K, we observe a drastic enhancement of the electron scattering rate, which aligns with the semiconducting-like property at high temperatures. These findings establish CsCr3Sb5 as a strongly correlated Hund’s metal with incipient flat bands near the Fermi level, which provides an electronic basis for understanding its novel properties compared to the weakly correlated AV3Sb5.
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Superconductivity in Trilayer Nickelate La4Ni3O10 under Pressure

Physical Review X American Physical Society (APS) 15:2 (2025) 021005

Authors:

Mingxin Zhang, Cuiying Pei, Di Peng, Xian Du, Weixiong Hu, Yantao Cao, Qi Wang, Juefei Wu, Yidian Li, Huanyu Liu, Chenhaoping Wen, Jing Song, Yi Zhao, Changhua Li, Weizheng Cao, Shihao Zhu, Qing Zhang, Na Yu, Peihong Cheng, Lili Zhang, Zhiwei Li, Jinkui Zhao, Yulin Chen, Changqing Jin, Hanjie Guo, Congjun Wu, Fan Yang, Qiaoshi Zeng, Shichao Yan, Lexian Yang, Yanpeng Qi
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