Electron correlation and incipient flat bands in the Kagome superconductor CsCr 3 Sb 5
Nature Communications Nature Research 16:1 (2025) 3229
Abstract:
Correlated kagome materials exhibit a compelling interplay between lattice geometry, electron correlation, and topology. In particular, the flat bands near the Fermi level provide a fertile playground for novel many-body states. Here we investigate the electronic structure of CsCr3Sb5 using high-resolution angle-resolved photoemission spectroscopy and ab-initio calculations. Our results suggest that Cr 3d electrons are intrinsically incoherent, showing strong electron correlation amplified by Hund’s coupling. Notably, we identify incipient flat bands close to the Fermi level, which are expected to significantly influence the electronic properties of the system. Across the density-wave-like transition at 55 K, we observe a drastic enhancement of the electron scattering rate, which aligns with the semiconducting-like property at high temperatures. These findings establish CsCr3Sb5 as a strongly correlated Hund’s metal with incipient flat bands near the Fermi level, which provides an electronic basis for understanding its novel properties compared to the weakly correlated AV3Sb5.Superconductivity in Trilayer Nickelate La4Ni3O10 under Pressure
Physical Review X American Physical Society (APS) 15:2 (2025) 021005
Dual topology and versatile Rashba-split surface state configurations in 2M-WS2 and 2M-WSe2
Physical Review B American Physical Society (APS) 111:11 (2025) 115151
Abstract:
The 2M-phase transition metal dichalcogenides have recently attracted intensive research interest due to their rich topological and superconducting phase diagrams. Apart from the topological surface states of 2M-WS2 near Γ that originated from the strong topological order, using angle-resolved photoemission spectroscopy, we discover additional Rashba-split states on the surfaces of both 2M-WS2 and 2M-WSe2, which extend in large momentum-energy regions. First-principles calculations well reproduce these states and attribute them to the weak topological orders. The calculations further indicate that the surface state connecting configurations are tunable under moderate pressure, suggesting that 2M-WS2 and WSe2 are promising platforms to study topological phase transition and explore topological superconductivity.Mott insulating phase and coherent-incoherent crossover across magnetic phase transition in 2D antiferromagnetic CrSBr
Science China Physics, Mechanics & Astronomy Springer Nature 68:6 (2025) ARTN 267411
Abstract:
In two-dimensional van der Waals magnetic materials, the interplay between magnetism and electron correlation can give rise to new ground states and lead to novel transport and optical properties. A fundamental question in these materials is how the electron correlation manifests and interacts with the magnetic orders. In this study, we demonstrate that the recently discovered 2D antiferromagnetic material, CrSBr is a Mott insulator, through the combined use of resonant and temperature-dependent angle-resolved photoemission spectroscopy techniques, supplemented by dynamical mean-field theory analysis. Intriguingly, we found that as the system transitions from the antiferromagnetic to the paramagnetic phases, its Mott bands undergo a reconfiguration, and a coherent-incoherent crossover, driven by the dissolution of the magnetic order. Our findings reveal a distinctive evolution of band structure associated with magnetic phase transitions, shedding light on the investigation of the intricate interplay between correlation and magnetic orders in strongly correlated van der Waals magnetic materials.Direct Visualization of the Impurity Occupancy Road Map in Ni-Substituted van der Waals Ferromagnet Fe<sub>3</sub>GaTe<sub>2</sub>.
Nano letters American Chemical Society (ACS) 25:11 (2025) 4260-4266