Electronic structures and photoemission spectroscopy

Abstract:

Using high-resolution angle-resolved photoemission spectroscopy (ARPES), we have mapped out the reconstructed electronic structure in the commensurate charge-density-wave (CDW) state of quasi-two-dimensional transition metal dichalcogenide 2H-TaSe2. The observation of the fine structure near Brillouin zone (BZ) center supplements the picture of Fermi surface folding in the 3×3 CDW state. In addition to the anisotropic CDW band gaps that energetically stabilize the system at the Fermi level in the first-order lock-in transition, we found band reconstruction at high binding energy, which can be well explained by the hybridization between main bands (MBs) and folded bands (FBs). Furthermore, in contrast to the perfectly nested quasi-one-dimensional system, triple-nesting-vector-induced CDW FBs increase the degeneracy of the band crossing and thus further enlarge the magnitude of band gap at certain momentum-energy positions. The visualization and modeling of CDW gaps in momentum-energy space reconciles the long-lasting controversy on the gap magnitude and suggests a weak-coupling Peierls physics in this system.

Abstract:

The original version of this Article contained an error in the spelling of the author Benjamin H. Williams, which was incorrectly given as Benjamin H. Willams. This has now been corrected in both the PDF and HTML versions of the Article.

Abstract:

We report on the electronic structure of the elemental topological semimetal α − Sn on InSb(001). High-resolution angle-resolved photoemission data allow us to observe the topological surface state (TSS) that is degenerate with the bulk band structure and show that the former is unaffected by different surface reconstructions. An unintentional p -type doping of the as-grown films was compensated by deposition of potassium or tellurium after the growth, thereby shifting the Dirac point of the surface state below the Fermi level. We show that, while having the potential to break time-reversal symmetry, iron impurities with a coverage of up to 0.25 monolayers do not have any further impact on the surface state beyond that of K or Te. Furthermore, we have measured the spin-momentum locking of electrons from the TSS by means of spin-resolved photoemission. Our results show that the spin vector lies fully in-plane, but it also has a finite radial component. Finally, we analyze the decay of photoholes introduced in the photoemission process, and by this gain insight into the many-body interactions in the system. Surprisingly, we extract quasiparticle lifetimes comparable to other topological materials where the TSS is located within a bulk band gap. We argue that the main decay of photoholes is caused by intraband scattering, while scattering into bulk states is suppressed due to different orbital symmetries of bulk and surface states.