Condensed Matter Theory

Abstract:

We study spectral statistics in spatially extended chaotic quantum many-body systems, using simple lattice Floquet models without time-reversal symmetry. Computing the spectral form factor $K(t)$ analytically and numerically, we show that it follows random matrix theory (RMT) at times longer than a many-body Thouless time, $t_{\rm Th}$. We obtain a striking dependence of $t_{\rm Th}$ on the spatial dimension $d$ and size of the system. For $d>1$, $t_{\rm Th}$ is finite in the thermodynamic limit and set by the inter-site coupling strength. By contrast, in one dimension $t_{\rm Th}$ diverges with system size, and for large systems there is a wide window in which spectral correlations are not of RMT form.

Abstract:

We analyze the effect of quenched disorder on spin-1/2 quantum magnets in which magnetic frustration promotes the formation of local singlets. Our results include a theory for 2D valence-bond solids subject to weak bond randomness, as well as extensions to stronger disorder regimes where we make connections with quantum spin liquids. We find, on various lattices, that the destruction of a valence-bond solid phase by weak quenched disorder leads inevitably to the nucleation of topological defects carrying spin-1/2 moments. This renormalizes the lattice into a strongly random spin network with interesting low-energy excitations. Similarly, when short-ranged valence bonds would be pinned by stronger disorder, we find that this putative glass is unstable to defects that carry spin-1/2 magnetic moments, and whose residual interactions decide the ultimate low-energy fate. Motivated by these results we conjecture Lieb-Schultz-Mattis-like restrictions on ground states for disordered magnets with spin 1/2 per statistical unit cell. These conjectures are supported by an argument for 1D spin chains. We apply insights from this study to the phenomenology of YbMgGaO4, a recently discovered triangular lattice spin-1/2 insulator which was proposed to be a quantum spin liquid. We instead explore a description based on the present theory. Experimental signatures, including unusual specific heat, thermal conductivity, and dynamical structure factor, and their behavior in a magnetic field, are predicted from the theory, and compare favorably with existing measurements on YbMgGaO4 and related materials.