Continuous-time multifarious systems. I. Equilibrium multifarious self-assembly

The Journal of Chemical Physics AIP Publishing 163:12 (2025) 124904

Authors:

Jakob Metson, Saeed Osat, Ramin Golestanian

Abstract:

Multifarious assembly models consider multiple structures assembled from a shared set of components, reflecting the efficient usage of components in biological self-assembly. These models are subject to a high-dimensional parameter space, with only a finite region of parameter space giving reliable self-assembly. Here, we use a continuous-time Gillespie simulation method to study multifarious self-assembly and find that the region of parameter space in which reliable self-assembly can be achieved is smaller than what was obtained previously using a discrete-time Monte Carlo simulation method. We explain this discrepancy through a detailed analysis of the stability of assembled structures against chimera formation. We find that our continuous-time simulations of multifarious self-assembly can expose this instability in large systems even at moderate simulation times. In contrast, discrete-time simulations are slow to show this instability, particularly for large system sizes. For the remaining state space, we find good agreement between the predictions of continuous- and discrete-time simulations. We present physical arguments that can help us predict the state boundaries in the parameter space and gain a deeper understanding of multifarious self-assembly.

Continuous-time multifarious systems. II. Non-reciprocal multifarious self-organization

The Journal of Chemical Physics AIP Publishing 163:12 (2025) 124905

Authors:

Jakob Metson, Saeed Osat, Ramin Golestanian

Abstract:

In the context of self-assembly, where complex structures can be assembled from smaller units, it is desirable to devise strategies toward disassembly and reassembly processes that reuse the constituent parts. A non-reciprocal multifarious self-organization strategy has been recently introduced and shown to have the capacity to exhibit this complex property. In this work, we study the model using continuous-time Gillespie simulations and compare the results against discrete-time Monte Carlo simulations investigated previously. Furthermore, using the continuous-time simulations, we explore important features in our system, namely, the nucleation time and interface growth velocity, which comprise the timescale of shape-shifting. We develop analytical calculations for the associated timescales and compare the results to those measured in simulations, allowing us to pin down the key mechanisms behind the observed timescales at different parameter values.

Quantum Hall Antidot as a Fractional Coulombmeter

preprint, arXiv:2509.04209

Authors:

Mario Di Luca, Emily Hajigeorgiou, Zekang Zhou, Tevž Lotrič, Tengyan Feng, Kenji Watanabe, Takashi Taniguchi, Steven H. Simon, Mitali Banerjee

Abstract:

The detection of fractionally charged quasiparticles, which arise in the fractional quantum Hall regime, is of fundamental importance for probing their exotic quantum properties. While electronic interferometers have been central to probe their statistical properties, their interpretation is often complicated by bulk-edge interactions. Antidots, potential hills in the quantum Hall regime, are particularly valuable in this context, as they overcome the geometric limitations of conventional designs and act as controlled impurities within a quantum point contact. Furthermore, antidots allow for quasiparticle charge detection through straightforward conductance measurements, replacing the need for more demanding techniques. In this work, we employ a gate-defined bilayer graphene antidot operating in the Coulomb-dominated regime to study quasiparticle tunneling in both integer and fractional quantum Hall states. We show that the gate-voltage period and the oscillation slope directly reveal the charge of the tunneling quasiparticles, providing a practical method to measure fractional charge in graphene. We report direct measurements of fractional charge, finding q=e/3 at ν=4/3, 5/3 and 7/3, q=2e/3 at ν=2/3 and q=3e/5 at ν=3/5, while at ν=8/3 we observe signatures of both e/3 and 2e/3 tunneling charge. The simplicity and tunability of this design open a pathway to extend antidot-based charge measurements to other van der Waals materials, establishing antidots as a powerful and broadly applicable platform to study the quantum Hall effect.

Quantum Hall Antidot as a Fractional Coulombmeter

(2025)

Authors:

Mario Di Luca, Emily Hajigeorgiou, Zekang Zhou, Tevž Lotrič, Tengyan Feng, Kenji Watanabe, Takashi Taniguchi, Steven H Simon, Mitali Banerjee

Putting a new spin on the incommensurate Kekulé spiral: from spin-valley locking and collective modes to fermiology and implications for superconductivity

(2025)

Authors:

Ziwei Wang, Glenn Wagner, Yves H Kwan, Nick Bultinck, Steven H Simon, SA Parameswaran