Condensed Matter Theory

Abstract:

The spontaneous (so-called Quincke) rotation of an uncharged, solid, dielectric, spherical particle under a steady uniform electric field is analyzed, accounting for the inertia of the particle and the transient fluid inertia, or “hydrodynamic memory,” due to the unsteady Stokes flow around the particle. The dynamics of the particle are encapsulated in three coupled nonlinear integro-differential equations for the evolution of the angular velocity of the particle, and the components of the induced dipole of the particle that are parallel and transverse to the applied field. These equations represent a generalization of the celebrated Lorenz system. A numerical solution of these ‘modified Lorenz equations’ (MLE) shows that hydrodynamic memory leads to an increase in the threshold field strength for chaotic particle rotation, which is in qualitative agreement with experimental observations. Furthermore, hydrodynamic memory leads to an increase in the range of field strengths where multistability between steady and chaotic rotation occurs. At large field strengths, chaos ceases, and the particle is predicted to execute periodic rotational motion.

Abstract:

We consider a nonlinear oscillator with state-dependent time-delay that displays a countably infinite number of nested limit cycle attractors, i.e. megastability. In the low-memory regime, the equation reduces to a self-excited nonlinear oscillator and we use averaging methods to analytically show quasilinear increasing amplitude of the megastable spectrum of quantized quasicircular orbits. We further assign a mechanical energy to each orbit using the Lyapunov energy function and obtain a quadratically increasing energy spectrum and (almost) constant frequency spectrum. We demonstrate transitions between different quantized orbits, i.e. different energy levels, by subjecting the system to an external finite-time harmonic driving. In the absence of external driving force, the oscillator asymptotes towards one of the megastable quantized orbits having a fixed average energy. For a large driving amplitude with frequency close to the limit cycle frequency, resonance drives transitions to higher energy levels. Alternatively, for large driving amplitude with frequency slightly detuned from limit-cycle frequency, beating effects can lead to transitions to lower energy levels. Such driven transitions between quantized orbits form a classical analog of quantum jumps. For excitations to higher energy levels, we show amplitude locking where nearby values of driving amplitudes result in the same response amplitude, i.e. the same final higher energy level. We rationalize this effect based on the basins of different limit cycles in phase space. From a practical viewpoint, our work might find applications in physical and engineering system where controlled transitions between several limit cycles of a multistable dynamical system is desired.

Abstract:

Magnetic heat capacity measurements of a high-quality single crystal of the dipole-octupole pyrochlore Ce2Hf2O7 down to a temperature of T=0.02 K are reported. These show a two-peaked structure, with a Schottky-like peak at T1∼0.065 K, similar to what is observed in its sister Ce pyrochlores Ce2Zr2O7 and Ce2Sn2O7. However, a second sharper peak is observed at T2∼0.025 K, signifying the entrance to the ground state. The ground state appears to have gapped excitations, as even the most abrupt extrapolation to CP=0 at T=0 K fully accounts for the Rln(2) entropy associated with the pseudospin-1/2 doublet for Ce3+ in this environment. The ground state could be conventionally ordered, although theory predicts a much larger anomaly in CP at much higher temperatures than the measured T2 for expectations from an all-in, all-out ground state of the XYZ Hamiltonian for Ce2Hf2O7. The sharp low-temperature peak could also signify a crossover from a classical spin liquid to a quantum spin liquid (QSL). For both scenarios, comparison of the measured CP with NLC calculations suggests that weak interactions beyond the nearest-neighbor XYZ Hamiltonian become relevant below T∼0.25 K. The diffuse magnetic neutron scattering observed from Ce2Hf2O7 at low temperatures between T2 and T1 resembles that observed from Ce2Zr2O7, which is well established as a π-flux quantum spin ice (QSI). Together with the peak in the heat capacity at T2, this diffuse scattering from Ce2Hf2O7 is suggestive of a classical spin liquid regime above T2 that is distinct from the zero-entropy quantum ground state below T2.